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Development of novel sub-ambient membrane systems for energy-efficient post-combustion CO2 capture

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  • Lee, Sunghoon
  • Yun, Seokwon
  • Kim, Jin-Kuk

Abstract

A substantial increase in CO2/N2 selectivity of the membrane under sub-ambient temperature conditions allows the design of CO2 capture processes in an energy-efficient and cost-effective manner. An innovative sub-ambient temperature membrane process is proposed in this study for the separation of CO2 from power plant flue gases, in which the high membrane selectivity is strategically utilized with the aid of a simple, external refrigeration cycle. In the new membrane process, a sweeping-integrated single membrane module integrated with a purification column is sufficient to achieve a high purity of 99.9% CO2 product with 90% CO2 recovery. Process optimization is utilized to determine cost-effective operating conditions and appropriate membrane configurations. The optimized sub-ambient temperature membrane process is shown to reduce the overall CO2 capture cost by 13% as well reducing the parasitic load by 16%, compared to a conventional multi-stage membrane process operated at ambient temperature conditions. The sensitivities of CO2 capture cost and energy with respect to key design variables such as pressure ratio, membrane performance (i.e. CO2 permeance and CO2/N2 selectivity) and CO2 recovery are investigated to provide conceptual insights and design guidelines for developing efficient membrane processes for the capture of CO2.

Suggested Citation

  • Lee, Sunghoon & Yun, Seokwon & Kim, Jin-Kuk, 2019. "Development of novel sub-ambient membrane systems for energy-efficient post-combustion CO2 capture," Applied Energy, Elsevier, vol. 238(C), pages 1060-1073.
  • Handle: RePEc:eee:appene:v:238:y:2019:i:c:p:1060-1073
    DOI: 10.1016/j.apenergy.2019.01.130
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    References listed on IDEAS

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    1. Luis Míguez, José & Porteiro, Jacobo & Pérez-Orozco, Raquel & Patiño, David & Rodríguez, Sandra, 2018. "Evolution of CO2 capture technology between 2007 and 2017 through the study of patent activity," Applied Energy, Elsevier, vol. 211(C), pages 1282-1296.
    2. Song, Chunfeng & Liu, Qingling & Ji, Na & Deng, Shuai & Zhao, Jun & Li, Yang & Kitamura, Yutaka, 2017. "Reducing the energy consumption of membrane-cryogenic hybrid CO2 capture by process optimization," Energy, Elsevier, vol. 124(C), pages 29-39.
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    Cited by:

    1. Fu, Hongming & Xue, Kaili & Li, Zhaohao & Zhang, Heng & Gao, Dan & Chen, Haiping, 2023. "Study on the performance of CO2 capture from flue gas with ceramic and PTFE membrane contactors," Energy, Elsevier, vol. 263(PA).
    2. Vo, Nguyen Dat & Oh, Dong Hoon & Kang, Jun-Ho & Oh, Min & Lee, Chang-Ha, 2020. "Dynamic-model-based artificial neural network for H2 recovery and CO2 capture from hydrogen tail gas," Applied Energy, Elsevier, vol. 273(C).
    3. Wen, Chuang & Li, Bo & Ding, Hongbing & Akrami, Mohammad & Zhang, Haoran & Yang, Yan, 2022. "Thermodynamics analysis of CO2 condensation in supersonic flows for the potential of clean offshore natural gas processing," Applied Energy, Elsevier, vol. 310(C).
    4. Pang, Ruizhi & Han, Yang & Chen, Kai K. & Yang, Yutong & Ho, W.S. Winston, 2022. "Matrimid substrates with bicontinuous surface and macrovoids in the bulk: A nearly ideal substrate for composite membranes in CO2 capture," Applied Energy, Elsevier, vol. 311(C).
    5. Lee, Sunghoon & Kim, Jin-Kuk, 2020. "Process-integrated design of a sub-ambient membrane process for CO2 removal from natural gas power plants," Applied Energy, Elsevier, vol. 260(C).
    6. Zhao, Yunlei & Jin, Bo & Luo, Xiao & Liang, Zhiwu, 2021. "Thermodynamic evaluation and experimental investigation of CaO-assisted Fe-based chemical looping reforming process for syngas production," Applied Energy, Elsevier, vol. 288(C).

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