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Experimental investigation of molten salt droplet quenching and solidification processes of heat recovery in thermochemical hydrogen production

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  • Ghandehariun, S.
  • Wang, Z.
  • Naterer, G.F.
  • Rosen, M.A.

Abstract

This paper investigates the heat transfer and X-ray diffraction patterns of solidified molten salt droplets in heat recovery processes of a thermochemical Cu–Cl cycle of hydrogen production. It is essential to recover the heat of the molten salt to enhance the overall thermal efficiency of the copper–chlorine cycle. A major portion of heat recovery within the cycle can be achieved by cooling and solidifying the molten salt exiting an oxygen reactor. Heat recovery from the molten salt is achieved by dispersing the molten stream into droplets. In this paper, an analytical study and experimental investigation of the thermal phenomena of a falling droplet quenched into water is presented, involving the droplet surface temperature during descent and resulting composition change in the quench process. The results show that it is feasible to quench the molten salt droplets for an efficient heat recovery process without introducing any material imbalance for the overall cycle integration.

Suggested Citation

  • Ghandehariun, S. & Wang, Z. & Naterer, G.F. & Rosen, M.A., 2015. "Experimental investigation of molten salt droplet quenching and solidification processes of heat recovery in thermochemical hydrogen production," Applied Energy, Elsevier, vol. 157(C), pages 267-275.
    • Handle: RePEc:eee:appene:v:157:y:2015:i:c:p:267-275
    DOI: 10.1016/j.apenergy.2015.08.002
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    Cited by:

    1. Zhuang, Rui & Wang, Xiaonan & Guo, Miao & Zhao, Yingru & El-Farra, Nael H. & Palazoglu, Ahmet, 2020. "Waste-to-hydrogen: Recycling HCl to produce H2 and Cl2," Applied Energy, Elsevier, vol. 259(C).
    2. Sadeghi, Shayan & Ghandehariun, Samane, 2022. "A standalone solar thermochemical water splitting hydrogen plant with high-temperature molten salt: Thermodynamic and economic analyses and multi-objective optimization," Energy, Elsevier, vol. 240(C).
    3. Sadeghi, Shayan & Ghandehariun, Samane & Rosen, Marc A., 2023. "Waste heat recovery potential in the thermochemical copper–chlorine cycle for hydrogen production: Development of an efficient and cost-effective heat exchanger network," Energy, Elsevier, vol. 282(C).
    4. Ofelia A. Jianu & Bharanidharan Rajasekaran, 2022. "Transient Thermo-Fluid Analysis of Free Falling CuCl and AgCl Droplets with Liquid-to-Solid Phase Change," Energies, MDPI, vol. 15(13), pages 1-14, June.

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