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Preliminary study on co-gasification behavior of deoiled asphalt with coal and biomass

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  • Zhang, Qian
  • Li, Qingfeng
  • Zhang, Linxian
  • Wang, Zhiqing
  • Jing, Xuliang
  • Yu, Zhongliang
  • Song, Shuangshuang
  • Fang, Yitian

Abstract

The co-gasification behavior of deoiled asphalt (DOA) with coal and biomass were investigated by a thermogravimetric analyzer (TGA). The gasification experiments were conducted under CO2 atmosphere within an isothermal temperature range from 900 to 1100°C. The physical properties of the samples were examined by X-ray diffraction (XRD), scanning electron microscopy–energy dispersive spectroscopy (SEM–EDS), N2 and CO2 adsorption and inductively coupled plasma-atomic emission spectrometry (ICP-AES). Compared with coal or biomass, the low surface area, high graphitization degree and the low ash content are the main reasons for the low reactivity of DOA. The co-gasification of coal and DOA does not show synergetic effect, while the combination of biomass and DOA shows higher gasification reactivity than that of being calculated. The synergetic effect is mainly caused by the alkali metals. Further study shows the transfer of the potassium from the surface of biomass to DOA greatly increases the active sites of the DOA, which leads to obvious improvement of the co-gasification reactions. Meanwhile, the gasification experiments of adding coal and biomass ashes to DOA also support the above explanations.

Suggested Citation

  • Zhang, Qian & Li, Qingfeng & Zhang, Linxian & Wang, Zhiqing & Jing, Xuliang & Yu, Zhongliang & Song, Shuangshuang & Fang, Yitian, 2014. "Preliminary study on co-gasification behavior of deoiled asphalt with coal and biomass," Applied Energy, Elsevier, vol. 132(C), pages 426-434.
    • Handle: RePEc:eee:appene:v:132:y:2014:i:c:p:426-434
    DOI: 10.1016/j.apenergy.2014.07.014
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    1. Oladejo, Jumoke M. & Adegbite, Stephen & Pang, Cheng Heng & Liu, Hao & Parvez, Ashak M. & Wu, Tao, 2017. "A novel index for the study of synergistic effects during the co-processing of coal and biomass," Applied Energy, Elsevier, vol. 188(C), pages 215-225.
    2. Zhang, Qian & Li, Qingfeng & Zhang, Linxian & Yu, Zhongliang & Jing, Xuliang & Wang, Zhiqing & Fang, Yitian & Huang, Wei, 2017. "Experimental study on co-pyrolysis and gasification of biomass with deoiled asphalt," Energy, Elsevier, vol. 134(C), pages 301-310.
    3. Li, Fenghai & Zhao, Chaoyue & Guo, Qianqian & Li, Yang & Fan, Hongli & Guo, Mingxi & Wu, Lishun & Huang, Jiejie & Fang, Yitian, 2020. "Exploration in ash-deposition (AD) behavior modification of low-rank coal by manure addition," Energy, Elsevier, vol. 208(C).
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    5. Oladejo, Jumoke & Adegbite, Stephen & Gao, Xiang & Liu, Hao & Wu, Tao, 2018. "Catalytic and non-catalytic synergistic effects and their individual contributions to improved combustion performance of coal/biomass blends," Applied Energy, Elsevier, vol. 211(C), pages 334-345.
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    7. Kamble, Alka D. & Mendhe, Vinod A. & Chavan, Prakash D. & Saxena, Vinod K., 2022. "Insights of mineral catalytic effects of high ash coal on carbon conversion in fluidized bed Co-gasification through FTIR, XRD, XRF and FE-SEM," Renewable Energy, Elsevier, vol. 183(C), pages 729-751.

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