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Experimental investigation of CO2–brine–rock interactions in relation with CO2 sequestration in an Iranian oil reservoir

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  • Rozita Akbari
  • Elnaz Khodapanah
  • Seyyed Alireza Tabatabaei‐Nezhad

Abstract

The main purpose of this study is to evaluate the feasibility of geologic CO2 sequestration in terms of CO2‐brine‐rock interactions in Ramin oil field, Iran. Static experiments were conducted with carbonate rocks at 70°C and atmospheric pressure for 14, 30, and 60 days. CO2‐brine‐rock interactions were inferred from the evaluation of Ca2+, Mg2+, Cl−, and SO42− concentrations and a thorough characterization of the carbonate rocks before and after treatment. Scanning electron microscopy (SEM) micrographs revealed the formation of dissolution pits and the growth of new structures. Energy dispersive X‐ray spectroscopy (EDS) and X‐ray diffraction (XRD) indicated these minerals to be calcite. Porosity of the carbonate rocks increased from an initial value of 4.72% to the maximum value of 11.83%. Then, it decreased to a value of 5.48% until the end of the experiments, that is, 60 days. Chemical analysis of brine suggested the precipitation and dissolution of calcium sulfate. In addition, dolomite dissolution and halite precipitation/dissolution were inferred. Calcite precipitation and porosity reduction suggested that CO2 can be stored via mineral entrapment in the Ramin oil field, which is desired from the perspective of CO2 geologic sequestration. © 2020 Society of Chemical Industry and John Wiley & Sons, Ltd.

Suggested Citation

  • Rozita Akbari & Elnaz Khodapanah & Seyyed Alireza Tabatabaei‐Nezhad, 2021. "Experimental investigation of CO2–brine–rock interactions in relation with CO2 sequestration in an Iranian oil reservoir," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(1), pages 69-80, February.
    • Handle: RePEc:wly:greenh:v:11:y:2021:i:1:p:69-80
    DOI: 10.1002/ghg.2032
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    References listed on IDEAS

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    1. Tiago A. Siqueira & Rodrigo S. Iglesias & J. Marcelo Ketzer, 2017. "Carbon dioxide injection in carbonate reservoirs – a review of CO 2 ‐water‐rock interaction studies," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 7(5), pages 802-816, October.
    2. Maldal, T & Tappel, I.M, 2004. "CO2 underground storage for Snøhvit gas field development," Energy, Elsevier, vol. 29(9), pages 1403-1411.
    3. Ghorbani, Afshin & Rahimpour, Hamid Reza & Ghasemi, Younes & Zoughi, Somayeh & Rahimpour, Mohammad Reza, 2014. "A Review of Carbon Capture and Sequestration in Iran: Microalgal Biofixation Potential in Iran," Renewable and Sustainable Energy Reviews, Elsevier, vol. 35(C), pages 73-100.
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    1. Huang, Qiang & Shen, Jian & Zhang, Bing & Zhao, Gang & Cheng, Ming & Cai, Ying & Li, Chao, 2023. "Real-time monitoring of coalbed methane production network following liquid CO2 injection in a low-efficiency well network: Response to gas and water production characteristics," Energy, Elsevier, vol. 285(C).

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