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Ultrafast X-ray probing of water structure below the homogeneous ice nucleation temperature

Author

Listed:
  • J. A. Sellberg

    (SUNCAT Center for Interface Science and Catalysis, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA
    AlbaNova University Center, Stockholm University, S-106 91 Stockholm, Sweden)

  • C. Huang

    (Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • T. A. McQueen

    (SUNCAT Center for Interface Science and Catalysis, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA
    Stanford University)

  • N. D. Loh

    (PULSE Institute, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA)

  • H. Laksmono

    (PULSE Institute, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA)

  • D. Schlesinger

    (AlbaNova University Center, Stockholm University, S-106 91 Stockholm, Sweden)

  • R. G. Sierra

    (PULSE Institute, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA)

  • D. Nordlund

    (Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • C. Y. Hampton

    (PULSE Institute, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA)

  • D. Starodub

    (PULSE Institute, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA)

  • D. P. DePonte

    (Center for Free-Electron Laser Science, DESY, Notkestrasse 85, 22607 Hamburg, Germany
    Linac Coherent Light Source, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • M. Beye

    (SUNCAT Center for Interface Science and Catalysis, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA
    Institute for Methods and Instrumentation in Synchrotron Radiation Research, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Wilhelm-Conrad-Röntgen Campus, Albert-Einstein-Strasse 15, 12489 Berlin, Germany)

  • C. Chen

    (SUNCAT Center for Interface Science and Catalysis, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA
    Stanford University)

  • A. V. Martin

    (Center for Free-Electron Laser Science, DESY, Notkestrasse 85, 22607 Hamburg, Germany)

  • A. Barty

    (Center for Free-Electron Laser Science, DESY, Notkestrasse 85, 22607 Hamburg, Germany)

  • K. T. Wikfeldt

    (AlbaNova University Center, Stockholm University, S-106 91 Stockholm, Sweden)

  • T. M. Weiss

    (Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • C. Caronna

    (Linac Coherent Light Source, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • J. Feldkamp

    (Linac Coherent Light Source, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • L. B. Skinner

    (Mineral Physics Institute, Stony Brook University, Stony Brook, New York, New York 11794-2100, USA)

  • M. M. Seibert

    (Linac Coherent Light Source, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • M. Messerschmidt

    (Linac Coherent Light Source, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • G. J. Williams

    (Linac Coherent Light Source, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • S. Boutet

    (Linac Coherent Light Source, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

  • L. G. M. Pettersson

    (AlbaNova University Center, Stockholm University, S-106 91 Stockholm, Sweden)

  • M. J. Bogan

    (PULSE Institute, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA)

  • A. Nilsson

    (SUNCAT Center for Interface Science and Catalysis, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025, USA
    AlbaNova University Center, Stockholm University, S-106 91 Stockholm, Sweden
    Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, PO Box 20450, Stanford, California 94309, USA)

Abstract

Femtosecond X-ray laser pulses are used to probe the structure of liquid water in micrometre-sized droplets that have been cooled below the homogeneous ice nucleation temperature, revealing the existence of metastable bulk liquid water down to temperatures of 227 kelvin.

Suggested Citation

  • J. A. Sellberg & C. Huang & T. A. McQueen & N. D. Loh & H. Laksmono & D. Schlesinger & R. G. Sierra & D. Nordlund & C. Y. Hampton & D. Starodub & D. P. DePonte & M. Beye & C. Chen & A. V. Martin & A. , 2014. "Ultrafast X-ray probing of water structure below the homogeneous ice nucleation temperature," Nature, Nature, vol. 510(7505), pages 381-384, June.
    • Handle: RePEc:nat:nature:v:510:y:2014:i:7505:d:10.1038_nature13266
    DOI: 10.1038/nature13266
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    Cited by:

    1. Guo, Dan & Cao, Xuewen & Ding, Gaoya & Zhang, Pan & Liu, Yang & Bian, Jiang, 2022. "Crystallization and nucleation mechanism of heavy hydrocarbons in natural gas," Energy, Elsevier, vol. 239(PB).

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