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Dual-comb spectroscopy based on quantum-cascade-laser frequency combs

Author

Listed:
  • Gustavo Villares

    (Institute for Quantum Electronics, ETH Zurich)

  • Andreas Hugi

    (Institute for Quantum Electronics, ETH Zurich)

  • Stéphane Blaser

    (Alpes Lasers SA, 1-3 Max.-de-Meuron, C.P. 1766)

  • Jérôme Faist

    (Institute for Quantum Electronics, ETH Zurich)

Abstract

Dual-comb spectroscopy performed in the mid-infrared—where molecules have their strongest rotovibrational absorption lines—offers the promise of high spectral resolution broadband spectroscopy with very short acquisition times (μs) and no moving parts. Recently, we demonstrated frequency comb operation of a quantum-cascade-laser. We now use that device in a compact, dual-comb spectrometer. The noise properties of the heterodyne beat are close to the shot noise limit. Broadband (15 cm−1) high-resolution (80 MHz) absorption spectroscopy of both a GaAs etalon and water vapour is demonstrated, showing the potential of quantum-cascade-laser frequency combs as the basis for a compact, all solid-state, broadband chemical sensor.

Suggested Citation

  • Gustavo Villares & Andreas Hugi & Stéphane Blaser & Jérôme Faist, 2014. "Dual-comb spectroscopy based on quantum-cascade-laser frequency combs," Nature Communications, Nature, vol. 5(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:5:y:2014:i:1:d:10.1038_ncomms6192
    DOI: 10.1038/ncomms6192
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    Cited by:

    1. Carolin P. Bauer & Zofia A. Bejm & Michelle K. Bollier & Justinas Pupeikis & Benjamin Willenberg & Ursula Keller & Christopher R. Phillips, 2024. "High-sensitivity dual-comb and cross-comb spectroscopy across the infrared using a widely tunable and free-running optical parametric oscillator," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    2. Borislav Hinkov & Florian Pilat & Laurin Lux & Patricia L. Souza & Mauro David & Andreas Schwaighofer & Daniela Ristanić & Benedikt Schwarz & Hermann Detz & Aaron M. Andrews & Bernhard Lendl & Gottfri, 2022. "A mid-infrared lab-on-a-chip for dynamic reaction monitoring," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    3. Prati, F. & Lugiato, L.A. & Gatti, A. & Columbo, L. & Silvestri, C. & Gioannini, M. & Brambilla, M. & Piccardo, M. & Capasso, F., 2021. "Global and localised temporal structures in driven ring quantum cascade lasers," Chaos, Solitons & Fractals, Elsevier, vol. 153(P1).
    4. Mingchen Liu & Robert M. Gray & Luis Costa & Charles R. Markus & Arkadev Roy & Alireza Marandi, 2023. "Mid-infrared cross-comb spectroscopy," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    5. Qiang Wang & Zhen Wang & Hui Zhang & Shoulin Jiang & Yingying Wang & Wei Jin & Wei Ren, 2022. "Dual-comb photothermal spectroscopy," Nature Communications, Nature, vol. 13(1), pages 1-7, December.

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