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Practical H2 supply from ammonia borane enabled by amorphous iron domain

Author

Listed:
  • Yufeng Chen

    (Soochow University)

  • Zhongling Lang

    (Northeast Normal University)

  • Kun Feng

    (Soochow University)

  • Kang Wang

    (Soochow University)

  • Yangguang Li

    (Northeast Normal University)

  • Zhenhui Kang

    (Soochow University)

  • Lin Guo

    (Beihang University)

  • Jun Zhong

    (Soochow University)

  • Jun Lu

    (Zhejiang University
    Quzhou Institute of Power Battery and Grid Energy Storage)

Abstract

Efficient catalysis of ammonia borane (AB) holds potential for realizing controlled energy release from hydrogen fuel and addressing cost challenges faced by hydrogen storage. Here, we report that amorphous domains on metallic Fe crystal structures (R-Fe2O3 Foam) can achieve AB catalytic performances and stability (turnover frequency (TOF) of 113.6 min−1, about 771 L H2 in 900 h, and 43.27 mL/(min·cm2) for 10×10 cm2 of Foam) that outperform reported benchmarks (most

Suggested Citation

  • Yufeng Chen & Zhongling Lang & Kun Feng & Kang Wang & Yangguang Li & Zhenhui Kang & Lin Guo & Jun Zhong & Jun Lu, 2024. "Practical H2 supply from ammonia borane enabled by amorphous iron domain," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-53574-x
    DOI: 10.1038/s41467-024-53574-x
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    References listed on IDEAS

    as
    1. Gunther Glenk & Stefan Reichelstein, 2019. "Publisher Correction: Economics of converting renewable power to hydrogen," Nature Energy, Nature, vol. 4(4), pages 347-347, April.
    2. Umit Bilge Demirci, 2020. "Ammonia Borane: An Extensively Studied, Though Not Yet Implemented, Hydrogen Carrier," Energies, MDPI, vol. 13(12), pages 1-45, June.
    3. Gunther Glenk & Stefan Reichelstein, 2019. "Economics of converting renewable power to hydrogen," Nature Energy, Nature, vol. 4(3), pages 216-222, March.
    4. Huan Yan & Yue Lin & Hong Wu & Wenhua Zhang & Zhihu Sun & Hao Cheng & Wei Liu & Chunlei Wang & Junjie Li & Xiaohui Huang & Tao Yao & Jinlong Yang & Shiqiang Wei & Junling Lu, 2017. "Bottom-up precise synthesis of stable platinum dimers on graphene," Nature Communications, Nature, vol. 8(1), pages 1-11, December.
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