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Boosting uranium extraction from Seawater by micro-redox reactors anchored in a seaweed-like adsorbent

Author

Listed:
  • Yinshan Zhang

    (East China University of Technology
    East China University of Technology)

  • Yingcai Wang

    (East China University of Technology)

  • Zhimin Dong

    (East China University of Technology
    East China University of Technology)

  • Youqun Wang

    (East China University of Technology
    East China University of Technology)

  • Yuhui Liu

    (East China University of Technology)

  • Xiaohong Cao

    (East China University of Technology)

  • Zhibin Zhang

    (East China University of Technology)

  • Chao Xu

    (Tsinghua University)

  • Ning Wang

    (State Key Laboratory of Marine Resource Utilization in South China Sea Hainan University)

  • Yunhai Liu

    (East China University of Technology
    East China University of Technology)

Abstract

Efficient extraction of uranium from seawater is expected to provide virtually infinite fuel sources to power nuclear reactors and thus enable sustainable development of nuclear energy. The extraction efficiency for uranium greatly depends on the availability of active adsorption sites on the adsorbents. Maximization of the utilization rate of the binding sites in the adsorbent is vital for improving adsorption capacity. Herein, micro-redox reactors functioned by Cu(I)/Cu(II) conversion are constructed internally in an adsorbent bearing both amidoxime and carboxyl groups to induce active regeneration of the inactivated binding sites to enhance uranium capture. This adsorbent has high adsorption capacity (962.40 mg-U/g-Ads), superior anti-fouling ability as well as excellent uranium uptake (14.62 mg-U/g-Ads) in natural seawater after 56 days, placing it at the top of high-performance sorbent materials for uranium harvest from seawater.

Suggested Citation

  • Yinshan Zhang & Yingcai Wang & Zhimin Dong & Youqun Wang & Yuhui Liu & Xiaohong Cao & Zhibin Zhang & Chao Xu & Ning Wang & Yunhai Liu, 2024. "Boosting uranium extraction from Seawater by micro-redox reactors anchored in a seaweed-like adsorbent," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-53366-3
    DOI: 10.1038/s41467-024-53366-3
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    References listed on IDEAS

    as
    1. Yihui Yuan & Qiuhan Yu & Meng Cao & Lijuan Feng & Shiwei Feng & Tingting Liu & Tiantian Feng & Bingjie Yan & Zhanhu Guo & Ning Wang, 2021. "Selective extraction of uranium from seawater with biofouling-resistant polymeric peptide," Nature Sustainability, Nature, vol. 4(8), pages 708-714, August.
    2. Zeyu Liu & Youshi Lan & Jianfeng Jia & Yiyun Geng & Xiaobin Dai & Litang Yan & Tongyang Hu & Jing Chen & Krzysztof Matyjaszewski & Gang Ye, 2022. "Multi-scale computer-aided design and photo-controlled macromolecular synthesis boosting uranium harvesting from seawater," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    3. Steven Chu & Arun Majumdar, 2012. "Opportunities and challenges for a sustainable energy future," Nature, Nature, vol. 488(7411), pages 294-303, August.
    4. Yihui Yuan & Tingting Liu & Juanxiu Xiao & Qiuhan Yu & Lijuan Feng & Biye Niu & Shiwei Feng & Jiacheng Zhang & Ning Wang, 2020. "DNA nano-pocket for ultra-selective uranyl extraction from seawater," Nature Communications, Nature, vol. 11(1), pages 1-8, December.
    5. Yizhou Dai & Huan Li & Chuanhao Wang & Weiqing Xue & Menglu Zhang & Donghao Zhao & Jing Xue & Jiawei Li & Laihao Luo & Chunxiao Liu & Xu Li & Peixin Cui & Qiu Jiang & Tingting Zheng & Songqi Gu & Yao , 2023. "Manipulating local coordination of copper single atom catalyst enables efficient CO2-to-CH4 conversion," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
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