IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v15y2024i1d10.1038_s41467-024-45564-w.html
   My bibliography  Save this article

Real-time tracking of coherent oscillations of electrons in a nanodevice by photo-assisted tunnelling

Author

Listed:
  • Yang Luo

    (Max Planck Institute for Solid State Research)

  • Frank Neubrech

    (Max Planck Institute for Solid State Research
    University of Stuttgart)

  • Alberto Martin-Jimenez

    (Max Planck Institute for Solid State Research)

  • Na Liu

    (Max Planck Institute for Solid State Research
    University of Stuttgart)

  • Klaus Kern

    (Max Planck Institute for Solid State Research
    Ecole Polytechnique Fédérale de Lausanne)

  • Manish Garg

    (Max Planck Institute for Solid State Research)

Abstract

Coherent collective oscillations of electrons excited in metallic nanostructures (localized surface plasmons) can confine incident light to atomic scales and enable strong light-matter interactions, which depend nonlinearly on the local field. Direct sampling of such collective electron oscillations in real-time is crucial to performing petahertz scale optical modulation, control, and readout in a quantum nanodevice. Here, we demonstrate real-time tracking of collective electron oscillations in an Au bowtie nanoantenna, by recording photo-assisted tunnelling currents generated by such oscillations in this quantum nanodevice. The collective electron oscillations show a noninstantaneous response to the driving laser fields with a T2 decay time of nearly 8 femtoseconds. The contributions of linear and nonlinear electron oscillations in the generated tunnelling currents were precisely determined. A phase control of electron oscillations in the nanodevice is illustrated. Functioning in ambient conditions, the excitation, phase control, and read-out of coherent electron oscillations pave the way toward on-chip light-wave electronics in quantum nanodevices.

Suggested Citation

  • Yang Luo & Frank Neubrech & Alberto Martin-Jimenez & Na Liu & Klaus Kern & Manish Garg, 2024. "Real-time tracking of coherent oscillations of electrons in a nanodevice by photo-assisted tunnelling," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-45564-w
    DOI: 10.1038/s41467-024-45564-w
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-024-45564-w
    File Function: Abstract
    Download Restriction: no
    File URL: https://libkey.io/10.1038/s41467-024-45564-w?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Yanan Dai & Zhikang Zhou & Atreyie Ghosh & Roger S. K. Mong & Atsushi Kubo & Chen-Bin Huang & Hrvoje Petek, 2020. "Plasmonic topological quasiparticle on the nanometre and femtosecond scales," Nature, Nature, vol. 588(7839), pages 616-619, December.
    2. R. Zhang & Y. Zhang & Z. C. Dong & S. Jiang & C. Zhang & L. G. Chen & L. Zhang & Y. Liao & J. Aizpurua & Y. Luo & J. L. Yang & J. G. Hou, 2013. "Chemical mapping of a single molecule by plasmon-enhanced Raman scattering," Nature, Nature, vol. 498(7452), pages 82-86, June.
    3. Michael Krüger & Markus Schenk & Peter Hommelhoff, 2011. "Attosecond control of electrons emitted from a nanoscale metal tip," Nature, Nature, vol. 475(7354), pages 78-81, July.
    4. M. Garg & M. Zhan & T. T. Luu & H. Lakhotia & T. Klostermann & A. Guggenmos & E. Goulielmakis, 2016. "Multi-petahertz electronic metrology," Nature, Nature, vol. 538(7625), pages 359-363, October.
    5. Yujia Yang & Marco Turchetti & Praful Vasireddy & William P. Putnam & Oliver Karnbach & Alberto Nardi & Franz X. Kärtner & Karl K. Berggren & Phillip D. Keathley, 2020. "Light phase detection with on-chip petahertz electronic networks," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    6. A. Sommer & E. M. Bothschafter & S. A. Sato & C. Jakubeit & T. Latka & O. Razskazovskaya & H. Fattahi & M. Jobst & W. Schweinberger & V. Shirvanyan & V. S. Yakovlev & R. Kienberger & K. Yabana & N. Ka, 2016. "Attosecond nonlinear polarization and light–matter energy transfer in solids," Nature, Nature, vol. 534(7605), pages 86-90, June.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Zhengyi Lu & Jiamin Ji & Haiming Ye & Hao Zhang & Shunping Zhang & Hongxing Xu, 2024. "Quantifying the ultimate limit of plasmonic near-field enhancement," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Jack Griffiths & Tamás Földes & Bart Nijs & Rohit Chikkaraddy & Demelza Wright & William M. Deacon & Dénes Berta & Charlie Readman & David-Benjamin Grys & Edina Rosta & Jeremy J. Baumberg, 2021. "Resolving sub-angstrom ambient motion through reconstruction from vibrational spectra," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    3. Linfei Li & Jeremy F. Schultz & Sayantan Mahapatra & Zhongyi Lu & Xu Zhang & Nan Jiang, 2022. "Chemically identifying single adatoms with single-bond sensitivity during oxidation reactions of borophene," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    4. Xiang-Dong Chen & En-Hui Wang & Long-Kun Shan & Ce Feng & Yu Zheng & Yang Dong & Guang-Can Guo & Fang-Wen Sun, 2021. "Focusing the electromagnetic field to 10−6λ for ultra-high enhancement of field-matter interaction," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    5. Jiří Doležal & Sofia Canola & Prokop Hapala & Rodrigo Cezar Campos Ferreira & Pablo Merino & Martin Švec, 2022. "Evidence of exciton-libron coupling in chirally adsorbed single molecules," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    6. M. Ossiander & K. Golyari & K. Scharl & L. Lehnert & F. Siegrist & J. P. Bürger & D. Zimin & J. A. Gessner & M. Weidman & I. Floss & V. Smejkal & S. Donsa & C. Lemell & F. Libisch & N. Karpowicz & J. , 2022. "The speed limit of optoelectronics," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    7. S. E. Ammerman & V. Jelic & Y. Wei & V. N. Breslin & M. Hassan & N. Everett & S. Lee & Q. Sun & C. A. Pignedoli & P. Ruffieux & R. Fasel & T. L. Cocker, 2021. "Lightwave-driven scanning tunnelling spectroscopy of atomically precise graphene nanoribbons," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    8. Victor Chang Lee & Lun Yue & Mette B. Gaarde & Yang-hao Chan & Diana Y. Qiu, 2024. "Many-body enhancement of high-harmonic generation in monolayer MoS2," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    9. Yaolong Li & Pengzuo Jiang & Xiaying Lyu & Xiaofang Li & Huixin Qi & Jinglin Tang & Zhaohang Xue & Hong Yang & Guowei Lu & Quan Sun & Xiaoyong Hu & Yunan Gao & Qihuang Gong, 2023. "Revealing low-loss dielectric near-field modes of hexagonal boron nitride by photoemission electron microscopy," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    10. Yang Luo & Shaoxiang Sheng & Michele Pisarra & Alberto Martin-Jimenez & Fernando Martin & Klaus Kern & Manish Garg, 2024. "Selective excitation of vibrations in a single molecule," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    11. Yang Luo & Alberto Martin-Jimenez & Michele Pisarra & Fernando Martin & Manish Garg & Klaus Kern, 2023. "Imaging and controlling coherent phonon wave packets in single graphene nanoribbons," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    12. Renming Liu & Ming Geng & Jindong Ai & Xinyi Fan & Zhixiang Liu & Yu-Wei Lu & Yanmin Kuang & Jing-Feng Liu & Lijun Guo & Lin Wu, 2024. "Deterministic positioning and alignment of a single-molecule exciton in plasmonic nanodimer for strong coupling," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    13. Hao He & Maofeng Cao & Yun Gao & Peng Zheng & Sen Yan & Jin-Hui Zhong & Lei Wang & Dayong Jin & Bin Ren, 2024. "Noise learning of instruments for high-contrast, high-resolution and fast hyperspectral microscopy and nanoscopy," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    14. Jan Reislöhner & Doyeong Kim & Ihar Babushkin & Adrian N. Pfeiffer, 2022. "Onset of Bloch oscillations in the almost-strong-field regime," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    15. Mingu Kang & Hyunwoo Kim & Elham Oleiki & Yeonjeong Koo & Hyeongwoo Lee & Huitae Joo & Jinseong Choi & Taeyong Eom & Geunsik Lee & Yung Doug Suh & Kyoung-Duck Park, 2022. "Conformational heterogeneity of molecules physisorbed on a gold surface at room temperature," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    16. Philip A. Thomas & Kishan S. Menghrajani & William L. Barnes, 2022. "All-optical control of phase singularities using strong light-matter coupling," Nature Communications, Nature, vol. 13(1), pages 1-6, December.
    17. Václav Hanus & Beatrix Fehér & Viktória Csajbók & Péter Sándor & Zsuzsanna Pápa & Judit Budai & Zilong Wang & Pallabi Paul & Adriana Szeghalmi & Péter Dombi, 2023. "Carrier-envelope phase on-chip scanner and control of laser beams," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-45564-w. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.