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Chemical mapping of a single molecule by plasmon-enhanced Raman scattering

Author

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  • R. Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • Y. Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • Z. C. Dong

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • S. Jiang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • C. Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • L. G. Chen

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • L. Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • Y. Liao

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • J. Aizpurua

    (Material Physics Center CSIC-UPV/EHU and Donostia International Physics Center DIPC, Paseo Manuel de Lardizabal 5, Donostia-San Sebastián 20018, Spain)

  • Y. Luo

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
    Theoretical Chemistry and Biology, School of Biotechnology, Royal Institute of Technology, S-10691 Stockholm, Sweden)

  • J. L. Yang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • J. G. Hou

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

Abstract

Chemical mapping of a single molecule by optical means down to subnanometre resolution is achieved by spectrally matching the resonance of a nanocavity plasmon to the vibronic transitions of the molecules being studied, using tip-enhanced Raman scattering.

Suggested Citation

  • R. Zhang & Y. Zhang & Z. C. Dong & S. Jiang & C. Zhang & L. G. Chen & L. Zhang & Y. Liao & J. Aizpurua & Y. Luo & J. L. Yang & J. G. Hou, 2013. "Chemical mapping of a single molecule by plasmon-enhanced Raman scattering," Nature, Nature, vol. 498(7452), pages 82-86, June.
    • Handle: RePEc:nat:nature:v:498:y:2013:i:7452:d:10.1038_nature12151
    DOI: 10.1038/nature12151
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    10. Linfei Li & Jeremy F. Schultz & Sayantan Mahapatra & Zhongyi Lu & Xu Zhang & Nan Jiang, 2022. "Chemically identifying single adatoms with single-bond sensitivity during oxidation reactions of borophene," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    11. S. E. Ammerman & V. Jelic & Y. Wei & V. N. Breslin & M. Hassan & N. Everett & S. Lee & Q. Sun & C. A. Pignedoli & P. Ruffieux & R. Fasel & T. L. Cocker, 2021. "Lightwave-driven scanning tunnelling spectroscopy of atomically precise graphene nanoribbons," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    12. Renming Liu & Ming Geng & Jindong Ai & Xinyi Fan & Zhixiang Liu & Yu-Wei Lu & Yanmin Kuang & Jing-Feng Liu & Lijun Guo & Lin Wu, 2024. "Deterministic positioning and alignment of a single-molecule exciton in plasmonic nanodimer for strong coupling," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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