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Chemical mapping of a single molecule by plasmon-enhanced Raman scattering

Author

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  • R. Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • Y. Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • Z. C. Dong

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • S. Jiang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • C. Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • L. G. Chen

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • L. Zhang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • Y. Liao

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • J. Aizpurua

    (Material Physics Center CSIC-UPV/EHU and Donostia International Physics Center DIPC, Paseo Manuel de Lardizabal 5, Donostia-San Sebastián 20018, Spain)

  • Y. Luo

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China
    Theoretical Chemistry and Biology, School of Biotechnology, Royal Institute of Technology, S-10691 Stockholm, Sweden)

  • J. L. Yang

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

  • J. G. Hou

    (Hefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, Anhui 230026, China)

Abstract

Chemical mapping of a single molecule by optical means down to subnanometre resolution is achieved by spectrally matching the resonance of a nanocavity plasmon to the vibronic transitions of the molecules being studied, using tip-enhanced Raman scattering.

Suggested Citation

  • R. Zhang & Y. Zhang & Z. C. Dong & S. Jiang & C. Zhang & L. G. Chen & L. Zhang & Y. Liao & J. Aizpurua & Y. Luo & J. L. Yang & J. G. Hou, 2013. "Chemical mapping of a single molecule by plasmon-enhanced Raman scattering," Nature, Nature, vol. 498(7452), pages 82-86, June.
    • Handle: RePEc:nat:nature:v:498:y:2013:i:7452:d:10.1038_nature12151
    DOI: 10.1038/nature12151
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    Cited by:

    1. Maxim Fatkullin & Dmitry Cheshev & Andrey Averkiev & Alina Gorbunova & Gennadiy Murastov & Jianxi Liu & Pavel Postnikov & Chong Cheng & Raul D. Rodriguez & Evgeniya Sheremet, 2024. "Photochemistry dominates over photothermal effects in the laser-induced reduction of graphene oxide by visible light," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
    2. Yang Luo & Shaoxiang Sheng & Michele Pisarra & Alberto Martin-Jimenez & Fernando Martin & Klaus Kern & Manish Garg, 2024. "Selective excitation of vibrations in a single molecule," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    3. Zhengyi Lu & Jiamin Ji & Haiming Ye & Hao Zhang & Shunping Zhang & Hongxing Xu, 2024. "Quantifying the ultimate limit of plasmonic near-field enhancement," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    4. Yang Luo & Alberto Martin-Jimenez & Michele Pisarra & Fernando Martin & Manish Garg & Klaus Kern, 2023. "Imaging and controlling coherent phonon wave packets in single graphene nanoribbons," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    5. Xiang-Dong Chen & En-Hui Wang & Long-Kun Shan & Ce Feng & Yu Zheng & Yang Dong & Guang-Can Guo & Fang-Wen Sun, 2021. "Focusing the electromagnetic field to 10−6λ for ultra-high enhancement of field-matter interaction," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
    6. S. E. Ammerman & V. Jelic & Y. Wei & V. N. Breslin & M. Hassan & N. Everett & S. Lee & Q. Sun & C. A. Pignedoli & P. Ruffieux & R. Fasel & T. L. Cocker, 2021. "Lightwave-driven scanning tunnelling spectroscopy of atomically precise graphene nanoribbons," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    7. Renming Liu & Ming Geng & Jindong Ai & Xinyi Fan & Zhixiang Liu & Yu-Wei Lu & Yanmin Kuang & Jing-Feng Liu & Lijun Guo & Lin Wu, 2024. "Deterministic positioning and alignment of a single-molecule exciton in plasmonic nanodimer for strong coupling," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    8. Hao He & Maofeng Cao & Yun Gao & Peng Zheng & Sen Yan & Jin-Hui Zhong & Lei Wang & Dayong Jin & Bin Ren, 2024. "Noise learning of instruments for high-contrast, high-resolution and fast hyperspectral microscopy and nanoscopy," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    9. Jiří Doležal & Sofia Canola & Prokop Hapala & Rodrigo Cezar Campos Ferreira & Pablo Merino & Martin Švec, 2022. "Evidence of exciton-libron coupling in chirally adsorbed single molecules," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    10. Yang Luo & Frank Neubrech & Alberto Martin-Jimenez & Na Liu & Klaus Kern & Manish Garg, 2024. "Real-time tracking of coherent oscillations of electrons in a nanodevice by photo-assisted tunnelling," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    11. Jack Griffiths & Tamás Földes & Bart Nijs & Rohit Chikkaraddy & Demelza Wright & William M. Deacon & Dénes Berta & Charlie Readman & David-Benjamin Grys & Edina Rosta & Jeremy J. Baumberg, 2021. "Resolving sub-angstrom ambient motion through reconstruction from vibrational spectra," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
    12. Mingu Kang & Hyunwoo Kim & Elham Oleiki & Yeonjeong Koo & Hyeongwoo Lee & Huitae Joo & Jinseong Choi & Taeyong Eom & Geunsik Lee & Yung Doug Suh & Kyoung-Duck Park, 2022. "Conformational heterogeneity of molecules physisorbed on a gold surface at room temperature," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    13. Linfei Li & Jeremy F. Schultz & Sayantan Mahapatra & Zhongyi Lu & Xu Zhang & Nan Jiang, 2022. "Chemically identifying single adatoms with single-bond sensitivity during oxidation reactions of borophene," Nature Communications, Nature, vol. 13(1), pages 1-9, December.

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