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Spin skyrmion gaps as signatures of strong-coupling insulators in magic-angle twisted bilayer graphene

Author

Listed:
  • Jiachen Yu

    (Stanford University
    Geballe Laboratory of Advanced Materials)

  • Benjamin A. Foutty

    (Geballe Laboratory of Advanced Materials
    Stanford University)

  • Yves H. Kwan

    (University of Oxford)

  • Mark E. Barber

    (Stanford University
    Geballe Laboratory of Advanced Materials)

  • Kenji Watanabe

    (National Institute for Materials Science, 1-1 Namiki)

  • Takashi Taniguchi

    (National Institute for Materials Science, 1-1 Namiki)

  • Zhi-Xun Shen

    (Stanford University
    Geballe Laboratory of Advanced Materials
    Stanford University
    Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory)

  • Siddharth A. Parameswaran

    (University of Oxford)

  • Benjamin E. Feldman

    (Geballe Laboratory of Advanced Materials
    Stanford University
    Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory)

Abstract

The flat electronic bands in magic-angle twisted bilayer graphene (MATBG) host a variety of correlated insulating ground states, many of which are predicted to support charged excitations with topologically non-trivial spin and/or valley skyrmion textures. However, it has remained challenging to experimentally address their ground state order and excitations, both because some of the proposed states do not couple directly to experimental probes, and because they are highly sensitive to spatial inhomogeneities in real samples. Here, using a scanning single-electron transistor, we observe thermodynamic gaps at even integer moiré filling factors at low magnetic fields. We find evidence of a field-tuned crossover from charged spin skyrmions to bare particle-like excitations, suggesting that the underlying ground state belongs to the manifold of strong-coupling insulators. From the spatial dependence of these states and the chemical potential variation within the flat bands, we infer a link between the stability of the correlated ground states and local twist angle and strain. Our work advances the microscopic understanding of the correlated insulators in MATBG and their unconventional excitations.

Suggested Citation

  • Jiachen Yu & Benjamin A. Foutty & Yves H. Kwan & Mark E. Barber & Kenji Watanabe & Takashi Taniguchi & Zhi-Xun Shen & Siddharth A. Parameswaran & Benjamin E. Feldman, 2023. "Spin skyrmion gaps as signatures of strong-coupling insulators in magic-angle twisted bilayer graphene," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-42275-6
    DOI: 10.1038/s41467-023-42275-6
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    References listed on IDEAS

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    1. Yu Saito & Fangyuan Yang & Jingyuan Ge & Xiaoxue Liu & Takashi Taniguchi & Kenji Watanabe & J. I. A. Li & Erez Berg & Andrea F. Young, 2021. "Isospin Pomeranchuk effect in twisted bilayer graphene," Nature, Nature, vol. 592(7853), pages 220-224, April.
    2. Asaf Rozen & Jeong Min Park & Uri Zondiner & Yuan Cao & Daniel Rodan-Legrain & Takashi Taniguchi & Kenji Watanabe & Yuval Oreg & Ady Stern & Erez Berg & Pablo Jarillo-Herrero & Shahal Ilani, 2021. "Entropic evidence for a Pomeranchuk effect in magic-angle graphene," Nature, Nature, vol. 592(7853), pages 214-219, April.
    3. Yuan Cao & Valla Fatemi & Shiang Fang & Kenji Watanabe & Takashi Taniguchi & Efthimios Kaxiras & Pablo Jarillo-Herrero, 2018. "Unconventional superconductivity in magic-angle graphene superlattices," Nature, Nature, vol. 556(7699), pages 43-50, April.
    4. Harpreet Singh Arora & Robert Polski & Yiran Zhang & Alex Thomson & Youngjoon Choi & Hyunjin Kim & Zhong Lin & Ilham Zaky Wilson & Xiaodong Xu & Jiun-Haw Chu & Kenji Watanabe & Takashi Taniguchi & Jas, 2020. "Superconductivity in metallic twisted bilayer graphene stabilized by WSe2," Nature, Nature, vol. 583(7816), pages 379-384, July.
    5. Xiaobo Lu & Petr Stepanov & Wei Yang & Ming Xie & Mohammed Ali Aamir & Ipsita Das & Carles Urgell & Kenji Watanabe & Takashi Taniguchi & Guangyu Zhang & Adrian Bachtold & Allan H. MacDonald & Dmitri K, 2019. "Superconductors, orbital magnets and correlated states in magic-angle bilayer graphene," Nature, Nature, vol. 574(7780), pages 653-657, October.
    6. Petr Stepanov & Ipsita Das & Xiaobo Lu & Ali Fahimniya & Kenji Watanabe & Takashi Taniguchi & Frank H. L. Koppens & Johannes Lischner & Leonid Levitov & Dmitri K. Efetov, 2020. "Untying the insulating and superconducting orders in magic-angle graphene," Nature, Nature, vol. 583(7816), pages 375-378, July.
    7. U. Zondiner & A. Rozen & D. Rodan-Legrain & Y. Cao & R. Queiroz & T. Taniguchi & K. Watanabe & Y. Oreg & F. Oppen & Ady Stern & E. Berg & P. Jarillo-Herrero & S. Ilani, 2020. "Cascade of phase transitions and Dirac revivals in magic-angle graphene," Nature, Nature, vol. 582(7811), pages 203-208, June.
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    Cited by:

    1. Jesse C. Hoke & Yifan Li & Julian May-Mann & Kenji Watanabe & Takashi Taniguchi & Barry Bradlyn & Taylor L. Hughes & Benjamin E. Feldman, 2024. "Uncovering the spin ordering in magic-angle graphene via edge state equilibration," Nature Communications, Nature, vol. 15(1), pages 1-7, December.

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