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Large area polymer semiconductor sub-microwire arrays by coaxial focused electrohydrodynamic jet printing for high-performance OFETs

Author

Listed:
  • Dazhi Wang

    (Dalian University of Technology
    Dalian University of Technology
    Ningbo Institute of Dalian University of Technology)

  • Liangkun Lu

    (Dalian University of Technology)

  • Zhiyuan Zhao

    (Beijing National Laboratory for Molecular Sciences, Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences)

  • Kuipeng Zhao

    (Dalian University of Technology)

  • Xiangyu Zhao

    (Dalian University of Technology)

  • Changchang Pu

    (Dalian University of Technology)

  • Yikang Li

    (Dalian University of Technology)

  • Pengfei Xu

    (Dalian University of Technology)

  • Xiangji Chen

    (Dalian University of Technology)

  • Yunlong Guo

    (Beijing National Laboratory for Molecular Sciences, Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences)

  • Liujia Suo

    (Dalian University of Technology)

  • Junsheng Liang

    (Dalian University of Technology)

  • Yan Cui

    (Dalian University of Technology)

  • Yunqi Liu

    (Beijing National Laboratory for Molecular Sciences, Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences)

Abstract

Large area and highly aligned polymer semiconductor sub-microwires were fabricated using the coaxial focused electrohydrodynamic jet printing technology. As indicated by the results, the sub-microwire arrays have smooth morphology, well reproducibility and controllable with a width of ~110 nm. Analysis shows that the molecular chains inside the sub-microwires mainly exhibited edge-on arrangement and the π-stacking direction (010) of the majority of crystals is parallel to the long axis of the sub-microwires. Sub-microwires based organic field effect transistors showed high mobility with an average of 1.9 cm2 V−1 s−1, approximately 5 times higher than that of thin film based organic field effect transistors. In addition, the number of sub-microwires can be conveniently controlled by the printing technique, which can subsequently concisely control the performance of organic field effect transistors. This work demonstrates that sub-microwires fabricated by the coaxial focused electrohydrodynamic jet printing technology create an alternative path for the applications of high-performance organic flexible device.

Suggested Citation

  • Dazhi Wang & Liangkun Lu & Zhiyuan Zhao & Kuipeng Zhao & Xiangyu Zhao & Changchang Pu & Yikang Li & Pengfei Xu & Xiangji Chen & Yunlong Guo & Liujia Suo & Junsheng Liang & Yan Cui & Yunqi Liu, 2022. "Large area polymer semiconductor sub-microwire arrays by coaxial focused electrohydrodynamic jet printing for high-performance OFETs," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-34015-z
    DOI: 10.1038/s41467-022-34015-z
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    References listed on IDEAS

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    1. Martin Kaltenbrunner & Tsuyoshi Sekitani & Jonathan Reeder & Tomoyuki Yokota & Kazunori Kuribara & Takeyoshi Tokuhara & Michael Drack & Reinhard Schwödiauer & Ingrid Graz & Simona Bauer-Gogonea & Sieg, 2013. "An ultra-lightweight design for imperceptible plastic electronics," Nature, Nature, vol. 499(7459), pages 458-463, July.
    2. Jie Liu & Hantang Zhang & Huanli Dong & Lingqiang Meng & Longfeng Jiang & Lang Jiang & Ying Wang & Junsheng Yu & Yanming Sun & Wenping Hu & Alan J. Heeger, 2015. "High mobility emissive organic semiconductor," Nature Communications, Nature, vol. 6(1), pages 1-8, December.
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