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Synthetic strategies of supported atomic clusters for heterogeneous catalysis

Author

Listed:
  • Hongpan Rong

    (School of Materials Science and Engineering, Beijing Institute of Technology)

  • Shufang Ji

    (Tsinghua University)

  • Jiatao Zhang

    (School of Materials Science and Engineering, Beijing Institute of Technology)

  • Dingsheng Wang

    (Tsinghua University)

  • Yadong Li

    (Tsinghua University)

Abstract

Supported atomic clusters with uniform metal sites and definite low-nuclearity are intermediate states between single-atom catalysts (SACs) and nanoparticles in size. Benefiting from the presence of metal–metal bonds, supported atomic clusters can trigger synergistic effects among every metal atom, which contributes to achieving unique catalytic properties different from SACs and nanoparticles. However, the scalable and precise synthesis and atomic-level insights into the structure–properties relationship of supported atomic clusters is a great challenge. This perspective presents the latest progress of the synthesis of supported atomic clusters, highlights how the structure affects catalytic properties, and discusses the limitations as well as prospects.

Suggested Citation

  • Hongpan Rong & Shufang Ji & Jiatao Zhang & Dingsheng Wang & Yadong Li, 2020. "Synthetic strategies of supported atomic clusters for heterogeneous catalysis," Nature Communications, Nature, vol. 11(1), pages 1-14, December.
    • Handle: RePEc:nat:natcom:v:11:y:2020:i:1:d:10.1038_s41467-020-19571-6
    DOI: 10.1038/s41467-020-19571-6
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    1. Qianhong Wang & Keng Sang & Changwei Liu & Zhihua Zhang & Wenyao Chen & Te Ji & Lina Li & Cheng Lian & Gang Qian & Jing Zhang & Xinggui Zhou & Weikang Yuan & Xuezhi Duan, 2024. "Nanoparticles as an antidote for poisoned gold single-atom catalysts in sustainable propylene epoxidation," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    2. Chenhui Zhou & Jia Shi & Zhaoqi Dong & Lingyou Zeng & Yan Chen & Ying Han & Lu Li & Wenyu Zhang & Qinghua Zhang & Lin Gu & Fan Lv & Mingchuan Luo & Shaojun Guo, 2024. "Oxophilic gallium single atoms bridged ruthenium clusters for practical anion-exchange membrane electrolyzer," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    3. Xinyi Yang & Wanqing Song & Kang Liao & Xiaoyang Wang & Xin Wang & Jinfeng Zhang & Haozhi Wang & Yanan Chen & Ning Yan & Xiaopeng Han & Jia Ding & Wenbin Hu, 2024. "Cohesive energy discrepancy drives the fabrication of multimetallic atomically dispersed materials for hydrogen evolution reaction," Nature Communications, Nature, vol. 15(1), pages 1-14, December.
    4. Yufei Zhao & Priyank V. Kumar & Xin Tan & Xinxin Lu & Xiaofeng Zhu & Junjie Jiang & Jian Pan & Shibo Xi & Hui Ying Yang & Zhipeng Ma & Tao Wan & Dewei Chu & Wenjie Jiang & Sean C. Smith & Rose Amal & , 2022. "Modulating Pt-O-Pt atomic clusters with isolated cobalt atoms for enhanced hydrogen evolution catalysis," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    5. Seung-Hee Ryu & Seungeun Kim & Hyunjoo Lee & Joon-Hwan Choi & Hojin Jeong, 2024. "Robust palladium oxide nano-cluster catalysts using atomic ions and strong interactions for high-performance methane oxidation," Nature Communications, Nature, vol. 15(1), pages 1-15, December.

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