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Highly efficient eco-friendly X-ray scintillators based on an organic manganese halide

Author

Listed:
  • Liang-Jin Xu

    (Florida State University)

  • Xinsong Lin

    (Florida State University)

  • Qingquan He

    (Florida State University)

  • Michael Worku

    (Florida State University)

  • Biwu Ma

    (Florida State University
    Florida State University)

Abstract

Scintillation based X-ray detection has received great attention for its application in a wide range of areas from security to healthcare. Here, we report highly efficient X-ray scintillators with state-of-the-art performance based on an organic metal halide, ethylenebis-triphenylphosphonium manganese (II) bromide ((C38H34P2)MnBr4), which can be prepared using a facile solution growth method at room temperature to form inch sized single crystals. This zero-dimensional organic metal halide hybrid exhibits green emission peaked at 517 nm with a photoluminescence quantum efficiency of ~ 95%. Its X-ray scintillation properties are characterized with an excellent linear response to X-ray dose rate, a high light yield of ~ 80,000 photon MeV−1, and a low detection limit of 72.8 nGy s−1. X-ray imaging tests show that scintillators based on (C38H34P2)MnBr4 powders provide an excellent visualization tool for X-ray radiography, and high resolution flexible scintillators can be fabricated by blending (C38H34P2)MnBr4 powders with polydimethylsiloxane.

Suggested Citation

  • Liang-Jin Xu & Xinsong Lin & Qingquan He & Michael Worku & Biwu Ma, 2020. "Highly efficient eco-friendly X-ray scintillators based on an organic manganese halide," Nature Communications, Nature, vol. 11(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:11:y:2020:i:1:d:10.1038_s41467-020-18119-y
    DOI: 10.1038/s41467-020-18119-y
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    Cited by:

    1. Ziwei Liu & Jingning Wu & Chen Cai & Bo Yang & Zhi-mei Qi, 2022. "Flexible hyperspectral surface plasmon resonance microscopy," Nature Communications, Nature, vol. 13(1), pages 1-15, December.
    2. Hailei Zhang & Bo Zhang & Chongyang Cai & Kaiming Zhang & Yu Wang & Yuan Wang & Yanmin Yang & Yonggang Wu & Xinwu Ba & Richard Hoogenboom, 2024. "Water-dispersible X-ray scintillators enabling coating and blending with polymer materials for multiple applications," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    3. Ansheng Luo & Jingru Zhang & Dongjie Xiao & Gaozhan Xie & Xinqi Xu & Qingxian Zhao & Chengxi Sun & Yanzhang Li & Zehua Zhang & Ping Li & Shouhua Luo & Xiaoji Xie & Qiming Peng & Huanhuan Li & Runfeng , 2024. "Efficient metal free organic radical scintillators," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    4. Enhai Song & Meihua Chen & Zitao Chen & Yayun Zhou & Weijie Zhou & Hong-Tao Sun & Xianfeng Yang & Jiulin Gan & Shi Ye & Qinyuan Zhang, 2022. "Mn2+-activated dual-wavelength emitting materials toward wearable optical fibre temperature sensor," Nature Communications, Nature, vol. 13(1), pages 1-9, December.

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