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Hydrogen Production from Water by Photolysis, Sonolysis and Sonophotolysis with Solid Solutions of Rare Earth, Gallium and Indium Oxides as Heterogeneous Catalysts

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  • Marta Penconi

    (Dipartimento di Chimica, Biologia e Biotecnologie, Università di Perugia, Via Elce di Sotto, 8, 06123 Perugia, Italy
    Current Affiliation: Instituto di Scienze e Tecnologie Molecolari del CNR (CNR-ISTM), via C. Golgi 19, 20133 Milano, Italy;)

  • Federico Rossi

    (Inter-University Research Center on Pollution and Environment "Mauro Felli" (CIRIAF), Via G. Duranti 67, 06125 Perugia, Italy)

  • Fausto Ortica

    (Dipartimento di Chimica, Biologia e Biotecnologie, Università di Perugia, Via Elce di Sotto, 8, 06123 Perugia, Italy
    Inter-University Research Center on Pollution and Environment "Mauro Felli" (CIRIAF), Via G. Duranti 67, 06125 Perugia, Italy
    Centre of Excellence on Nanostructured Innovative Materials (CEMIN), Università di Perugia, via Elce di Sotto 8, 06123 Perugia, Italy
    Istituto Nazionale di Fisica Nucleare (INFN), Sezione di Perugia, Via Pascoli, 06123 Perugia, Italy)

  • Fausto Elisei

    (Dipartimento di Chimica, Biologia e Biotecnologie, Università di Perugia, Via Elce di Sotto, 8, 06123 Perugia, Italy
    Inter-University Research Center on Pollution and Environment "Mauro Felli" (CIRIAF), Via G. Duranti 67, 06125 Perugia, Italy
    Centre of Excellence on Nanostructured Innovative Materials (CEMIN), Università di Perugia, via Elce di Sotto 8, 06123 Perugia, Italy)

  • Pier Luigi Gentili

    (Dipartimento di Chimica, Biologia e Biotecnologie, Università di Perugia, Via Elce di Sotto, 8, 06123 Perugia, Italy
    Inter-University Research Center on Pollution and Environment "Mauro Felli" (CIRIAF), Via G. Duranti 67, 06125 Perugia, Italy)

Abstract

In this work, we present the hydrogen production by photolysis, sonolysis and sonophotolysis of water in the presence of newly synthesized solid solutions of rare earth, gallium and indium oxides playing as catalysts. From the experiments of photolysis, we found that the best photocatalyst is the solid solution Y 0.8 Ga 0.2 InO 3 doped by sulphur atoms. In experiments of sonolysis, we optimized the rate of hydrogen production by changing the amount of water, adding ethanol and tuning the power of our piezoelectric transducer. Finally, we performed sonolysis and sonophotolysis experiments in the presence of S:Y 0.8 Ga 0.2 InO 3 finding a promising synergistic effect of UV-visible electromagnetic waves and 38 kHz ultrasound waves in producing H 2 .

Suggested Citation

  • Marta Penconi & Federico Rossi & Fausto Ortica & Fausto Elisei & Pier Luigi Gentili, 2015. "Hydrogen Production from Water by Photolysis, Sonolysis and Sonophotolysis with Solid Solutions of Rare Earth, Gallium and Indium Oxides as Heterogeneous Catalysts," Sustainability, MDPI, vol. 7(7), pages 1-16, July.
    • Handle: RePEc:gam:jsusta:v:7:y:2015:i:7:p:9310-9325:d:52661
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    References listed on IDEAS

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    1. Sarkar, Nibedita & Ghosh, Sumanta Kumar & Bannerjee, Satarupa & Aikat, Kaustav, 2012. "Bioethanol production from agricultural wastes: An overview," Renewable Energy, Elsevier, vol. 37(1), pages 19-27.
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