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Innovative Technological Approach for the Cyclic Nutrients Adsorption by Post-Digestion Sewage Sludge-Based Ash Co-Formed with Some Nanostructural Additives under a Circular Economy Framework

Author

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  • Piotr Sakiewicz

    (Division of Nanocrystalline and Functional Materials and Sustainable Pro-Ecological Technologies, Institute of Engineering Materials and Biomaterials, Faculty of Mechanical Engineering, Silesian University of Technology, Konarskiego 18A, 44-100 Gliwice, Poland)

  • Krzysztof Piotrowski

    (Department of Chemical Engineering and Process Design, Faculty of Chemistry, Silesian University of Technology, ks. M. Strzody 7, 44-100 Gliwice, Poland)

  • Mariola Rajca

    (Institute of Water and Wastewater Engineering, Faculty of Energy and Environmental Engineering, Silesian University of Technology, Konarskiego 18, 44-100 Gliwice, Poland)

  • Izabella Maj

    (Department of Power Engineering and Turbomachinery, Faculty of Energy and Environmental Engineering, Silesian University of Technology, Konarskiego 18, 44-100 Gliwice, Poland)

  • Sylwester Kalisz

    (Department of Power Engineering and Turbomachinery, Faculty of Energy and Environmental Engineering, Silesian University of Technology, Konarskiego 18, 44-100 Gliwice, Poland)

  • Józef Ober

    (Department of Applied Social Sciences, Faculty of Organization and Management, Silesian University of Technology, Roosevelta 26-28, 41-800 Zabrze, Poland)

  • Janusz Karwot

    (Sewage and Water Supply Ltd., Pod Lasem 62, 44-210 Rybnik, Poland)

  • Krishna R. Pagilla

    (Department of Civil & Environmental Engineering, University of Nevada, Reno, NV 89557, USA)

Abstract

This paper presents a new, innovative technological approach, in line with Circular Economy principles, to the effective management of sludge generated during municipal wastewater treatment processes and subsequently used for biogas production. This approach allows for optimal, functional, and controlled cascade-type biotechnological thermal conversion of carbon compounds present in sewage sludge, later in solid digestate residues (after biogas production), and finally in the ash structure (after incineration, purposefully dosed nanostructural additives make the production of a useful solid product possible, especially for cyclic adsorption and slow release of nutrients (N, P, K) in the soil). The idea is generally targeted at achieving an innovative conversion cycle under a Circular Economy framework. In particular, it is based on an energy carrier (methane biogas) and direct energy production. The functionalized combustion by-products can be advantageous in agriculture. The use of ashes with nanostructural additives (halloysite, kaolinite) from combustion of sewage sludge after the anaerobic fermentation as an adsorbent of selected nutrients important in agriculture (Na + , K + , NO 3 − , SO 4 2− , PO 4 3− , Cl − ) was verified at laboratory scale. The tests were carried out both for pure ash and for the ash derived from combustion with the purposeful addition of kaolinite or halloysite. The equilibrium conditions for nitrate, potassium, sodium, phosphate(V), sulphate(VI), and chloride ions from aqueous solutions with the use of the three adsorbent structures were determined. The obtained innovative results were interpreted theoretically with adsorption isotherm models (Langmuir, Freundlich, Temkin, Jovanović). The most spectacular and clearly favorable results related to the influence of nanostructural additives in the process of sludge combustion, and formation of sorption surfaces under high temperature conditions were identified in the case of sorption-based separation of phosphate(V) ions (an increase from 1.13% to 61.24% with the addition of kaolinite, and even up to 76.19% with addition of halloysite).

Suggested Citation

  • Piotr Sakiewicz & Krzysztof Piotrowski & Mariola Rajca & Izabella Maj & Sylwester Kalisz & Józef Ober & Janusz Karwot & Krishna R. Pagilla, 2022. "Innovative Technological Approach for the Cyclic Nutrients Adsorption by Post-Digestion Sewage Sludge-Based Ash Co-Formed with Some Nanostructural Additives under a Circular Economy Framework," IJERPH, MDPI, vol. 19(17), pages 1-28, September.
    • Handle: RePEc:gam:jijerp:v:19:y:2022:i:17:p:11119-:d:907038
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    References listed on IDEAS

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    1. Jarosław Brodny & Magdalena Tutak & Peter Bindzár, 2021. "Assessing the Level of Renewable Energy Development in the European Union Member States. A 10-Year Perspective," Energies, MDPI, vol. 14(13), pages 1-38, June.
    2. Sakiewicz, P. & Piotrowski, K. & Ober, J. & Karwot, J., 2020. "Innovative artificial neural network approach for integrated biogas – wastewater treatment system modelling: Effect of plant operating parameters on process intensification," Renewable and Sustainable Energy Reviews, Elsevier, vol. 124(C).
    3. Andreas Nordin & Anna Strandberg & Sana Elbashir & Lars-Erik Åmand & Nils Skoglund & Anita Pettersson, 2020. "Co-Combustion of Municipal Sewage Sludge and Biomass in a Grate Fired Boiler for Phosphorus Recovery in Bottom Ash," Energies, MDPI, vol. 13(7), pages 1-24, April.
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    10. Sakiewicz, Piotr & Piotrowski, Krzysztof & Kalisz, Sylwester, 2020. "Neural network prediction of parameters of biomass ashes, reused within the circular economy frame," Renewable Energy, Elsevier, vol. 162(C), pages 743-753.
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    Cited by:

    1. Kamila Vávrová & Tomas Králík & Lukáš Janota & Olga Šolcová & Milan Čárský & Karel Soukup & Miroslav Vítek, 2023. "Process Economy of Alternative Fuel Production from Sewage Sludge and Waste Celluloses Biomass," Energies, MDPI, vol. 16(1), pages 1-12, January.
    2. Izabella Maj, 2022. "Significance and Challenges of Poultry Litter and Cattle Manure as Sustainable Fuels: A Review," Energies, MDPI, vol. 15(23), pages 1-17, November.
    3. Izabella Maj & Krzysztof Matus, 2023. "Aluminosilicate Clay Minerals: Kaolin, Bentonite, and Halloysite as Fuel Additives for Thermal Conversion of Biomass and Waste," Energies, MDPI, vol. 16(11), pages 1-17, May.
    4. Jaros³aw Brodny & Magdalena Tutak, 2023. "The level of implementing sustainable development goal "Industry, innovation and infrastructure" of Agenda 2030 in the European Union countries: Application of MCDM methods," Oeconomia Copernicana, Institute of Economic Research, vol. 14(1), pages 47-102, March.

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