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Steam Gasification of Torrefied/Carbonized Wheat Straw for H 2 -Enriched Syngas Production and Tar Reduction

Author

Listed:
  • Kejie Wang

    (Engineering Laboratory for AgroBiomass Recycling & Valorizing, College of Engineering, China Agricultural University, Beijing 100083, China
    These authors contributed equally to this work.)

  • Ge Kong

    (Engineering Laboratory for AgroBiomass Recycling & Valorizing, College of Engineering, China Agricultural University, Beijing 100083, China
    These authors contributed equally to this work.)

  • Guanyu Zhang

    (Engineering Laboratory for AgroBiomass Recycling & Valorizing, College of Engineering, China Agricultural University, Beijing 100083, China)

  • Xin Zhang

    (Engineering Laboratory for AgroBiomass Recycling & Valorizing, College of Engineering, China Agricultural University, Beijing 100083, China)

  • Lujia Han

    (Engineering Laboratory for AgroBiomass Recycling & Valorizing, College of Engineering, China Agricultural University, Beijing 100083, China)

  • Xuesong Zhang

    (Engineering Laboratory for AgroBiomass Recycling & Valorizing, College of Engineering, China Agricultural University, Beijing 100083, China)

Abstract

Torrefaction/carbonization integrated with steam gasification of agricultural biomass for gas production and tar reduction was not investigated. The aim of this study was to evaluate the influence of the torrefaction/carbonization severity on H 2 -enriched syngas production and tar reduction during steam gasification of wheat straw (WS). The torrefaction/carbonization experiments were initially performed at 220–500 °C to examine the effect of pretreated temperature on the fuel properties of torrefied/carbonized WS. Then, the gasification temperature (700–900 °C) was optimized at 900 °C in terms of gas formation behaviors. Afterward, steam gasification of raw and torrefied/carbonized WS feedstocks was conducted. WS carbonized at 500 °C (WS-500) possessed the highest H 2 concentration (54.21 vol%) and syngas purity (85.59%), while the maximum H 2 /CO molar ratio (1.83), high carbon conversion efficiency (90.33 C%) and cold gas efficiency (109.24%) were observed for WS torrefied at 280 °C. Notably, the cumulative gas yield, H 2 yield, and syngas yield respectively reached 102.68 mmol/g, 55.66 mmol/g, and 87.89 mmol/g from steam gasification of WS-500. In addition, the carbonized WS feedstocks, especially WS-500, revealed a lower tar content. Simply put, integrating torrefaction/carbonization with steam gasification provided a novel and effective route to manufacture H 2 -enriched syngas with extremely low tar content from agricultural biomass.

Suggested Citation

  • Kejie Wang & Ge Kong & Guanyu Zhang & Xin Zhang & Lujia Han & Xuesong Zhang, 2022. "Steam Gasification of Torrefied/Carbonized Wheat Straw for H 2 -Enriched Syngas Production and Tar Reduction," IJERPH, MDPI, vol. 19(17), pages 1-15, August.
    • Handle: RePEc:gam:jijerp:v:19:y:2022:i:17:p:10475-:d:895162
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    References listed on IDEAS

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    1. Sergey M. Frolov & Anton S. Silantiev & Ilias A. Sadykov & Viktor A. Smetanyuk & Fedor S. Frolov & Jaroslav K. Hasiak & Alexey B. Vorob’ev & Alexey V. Inozemtsev & Jaroslav O. Inozemtsev, 2023. "Gasification of Waste Machine Oil by the Ultra-Superheated Mixture of Steam and Carbon Dioxide," Waste, MDPI, vol. 1(2), pages 1-17, June.
    2. Kong, Ge & Zhang, Xin & Wang, Kejie & Zhou, Linling & Wang, Jin & Zhang, Xuesong & Han, Lujia, 2023. "Tunable H2/CO syngas production from co-gasification integrated with steam reforming of sewage sludge and agricultural biomass: A experimental study," Applied Energy, Elsevier, vol. 342(C).
    3. Sergey M. Frolov, 2022. "Organic Waste Gasification by Ultra-Superheated Steam," Energies, MDPI, vol. 16(1), pages 1-11, December.
    4. Sergey M. Frolov & Konstantin S. Panin & Viktor A. Smetanyuk, 2024. "Gasification of Liquid Hydrocarbon Waste by the Ultra-Superheated Mixture of Steam and Carbon Dioxide: A Thermodynamic Study," Energies, MDPI, vol. 17(9), pages 1-20, April.

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