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Hydrogen Storage in Pristine and d10-Block Metal-Anchored Activated Carbon Made from Local Wastes

Author

Listed:
  • Mohamed F. Aly Aboud

    (Sustainable Energy Technologies Center, College of Engineering, King Saud University, P.O. Box 800, Riyadh 11421, Saudi Arabia
    Mining, Metallurgical and Petroleum Engineering Department, Faculty of Engineering, Al-Azhar University, Nasr City, Cairo 11371, Egypt)

  • Zeid A. ALOthman

    (Advanced Materials Research Chair, Chemistry Department, P.O. Box 2455, College of Science, King Saud University, Riyadh 11451, Saudi Arabia)

  • Mohamed A. Habila

    (Advanced Materials Research Chair, Chemistry Department, P.O. Box 2455, College of Science, King Saud University, Riyadh 11451, Saudi Arabia)

  • Claudia Zlotea

    (ICMPE/CNRS-UPEC, UMR 7182, 2-8 rue Henri Dunant, 94320 Thiais, France)

  • Michel Latroche

    (ICMPE/CNRS-UPEC, UMR 7182, 2-8 rue Henri Dunant, 94320 Thiais, France)

  • Fermin Cuevas

    (ICMPE/CNRS-UPEC, UMR 7182, 2-8 rue Henri Dunant, 94320 Thiais, France)

Abstract

Activated carbon has been synthesized from local palm shell, cardboard and plastics municipal waste in the Kingdom of Saudi Arabia. It exhibits a surface area of 930 m 2 /g and total pore volume of 0.42 cm 3 /g. This pristine activated carbon has been further anchored with nickel, palladium and platinum metal particles by ultrasound-assisted impregnation. Deposition of nanosized Pt particles as small as 3 nm has been achieved, while for Ni and Pd their size reaches 100 nm. The solid-gas hydrogenation properties of the pristine and metal-anchored activated carbon have been determined. The pristine material exhibits a reversible hydrogen storage capacity of 2.3 wt% at 77 K and 3 MPa which is higher than for the doped ones. In these materials, the spillover effect due to metal doping is of minor importance in enhancing the hydrogen uptake compared with the counter-effect of the additional mass of the metal particles and pore blocking on the carbon surface.

Suggested Citation

  • Mohamed F. Aly Aboud & Zeid A. ALOthman & Mohamed A. Habila & Claudia Zlotea & Michel Latroche & Fermin Cuevas, 2015. "Hydrogen Storage in Pristine and d10-Block Metal-Anchored Activated Carbon Made from Local Wastes," Energies, MDPI, vol. 8(5), pages 1-13, April.
  • Handle: RePEc:gam:jeners:v:8:y:2015:i:5:p:3578-3590:d:48883
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    References listed on IDEAS

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    1. E. D. Minot & Yuval Yaish & Vera Sazonova & Paul L. McEuen, 2004. "Determination of electron orbital magnetic moments in carbon nanotubes," Nature, Nature, vol. 428(6982), pages 536-539, April.
    2. Midilli, A. & Ay, M. & Dincer, I. & Rosen, M. A., 2005. "On hydrogen and hydrogen energy strategies: I: current status and needs," Renewable and Sustainable Energy Reviews, Elsevier, vol. 9(3), pages 255-271, June.
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    Cited by:

    1. Craig M. Jensen & Etsuo Akiba & Hai-Wen Li, 2016. "Hydrides: Fundamentals and Applications," Energies, MDPI, vol. 9(4), pages 1-2, April.
    2. Vincenzo Palma & Concetta Ruocco & Eugenio Meloni & Antonio Ricca, 2017. "Influence of Catalytic Formulation and Operative Conditions on Coke Deposition over CeO 2 -SiO 2 Based Catalysts for Ethanol Reforming," Energies, MDPI, vol. 10(7), pages 1-13, July.

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