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Non-Catalytic Partial Oxidation of Hydrocarbon Gases to Syngas and Hydrogen: A Systematic Review

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  • Iren A. Makaryan

    (Federal Research Center of Problems of Chemical Physics and Medicinal Chemistry, Russian Academy of Sciences, Ac. Semenov av. 1, 142432 Chernogolovka, Russia)

  • Eugene A. Salgansky

    (Federal Research Center of Problems of Chemical Physics and Medicinal Chemistry, Russian Academy of Sciences, Ac. Semenov av. 1, 142432 Chernogolovka, Russia)

  • Vladimir S. Arutyunov

    (Federal Research Center of Problems of Chemical Physics and Medicinal Chemistry, Russian Academy of Sciences, Ac. Semenov av. 1, 142432 Chernogolovka, Russia
    N. N. Semenov Federal Research Center for Chemical Physics, Russian Academy of Sciences, 119991 Moscow, Russia)

  • Igor V. Sedov

    (Federal Research Center of Problems of Chemical Physics and Medicinal Chemistry, Russian Academy of Sciences, Ac. Semenov av. 1, 142432 Chernogolovka, Russia)

Abstract

The review contains a comparative analysis of studies on the production of hydrogen and syngas based on the processes of partial oxidation of natural gas and other types of gas feedstock. The results presented in the literature show the high potential of non-catalytic autothermal processes of partial oxidation of hydrocarbons for the development of gas chemistry and energetics. The partial oxidation of hydrocarbons makes it possible to overcome such serious shortcomings of traditional syngas production technologies as technological complexity and high energy and capital intensity. The features of non-catalytic partial oxidation of hydrocarbon gases, the obtained experimental results and the results of kinetic modeling of various options for the implementation of the process, which confirm the adequacy of the kinetic mechanisms used for the analysis, are considered in detail. Examples of industrial implementation of processes based on partial oxidation and proposed alternative options for its organization are considered. Designs of reactors used to ensure stable conversion of rich mixtures of hydrocarbons with an oxidizer are presented. The possibility of obtaining other chemical products by partial oxidation of hydrocarbons is discussed.

Suggested Citation

  • Iren A. Makaryan & Eugene A. Salgansky & Vladimir S. Arutyunov & Igor V. Sedov, 2023. "Non-Catalytic Partial Oxidation of Hydrocarbon Gases to Syngas and Hydrogen: A Systematic Review," Energies, MDPI, vol. 16(6), pages 1-23, March.
    • Handle: RePEc:gam:jeners:v:16:y:2023:i:6:p:2916-:d:1104176
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    References listed on IDEAS

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    1. Iren A. Makaryan & Igor V. Sedov & Eugene A. Salgansky & Artem V. Arutyunov & Vladimir S. Arutyunov, 2022. "A Comprehensive Review on the Prospects of Using Hydrogen–Methane Blends: Challenges and Opportunities," Energies, MDPI, vol. 15(6), pages 1-27, March.
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    Cited by:

    1. Alessandra Di Nardo & Marcella Calabrese & Virginia Venezia & Maria Portarapillo & Maria Turco & Almerinda Di Benedetto & Giuseppina Luciani, 2023. "Addressing Environmental Challenges: The Role of Hydrogen Technologies in a Sustainable Future," Energies, MDPI, vol. 16(23), pages 1-29, December.
    2. Mattia Boscherini & Alba Storione & Matteo Minelli & Francesco Miccio & Ferruccio Doghieri, 2023. "New Perspectives on Catalytic Hydrogen Production by the Reforming, Partial Oxidation and Decomposition of Methane and Biogas," Energies, MDPI, vol. 16(17), pages 1-33, September.

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