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A Comparative Study of Equivalent Circuit Models for Electro-Chemical Impedance Spectroscopy Analysis of Proton Exchange Membrane Fuel Cells

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  • Lei Zhao

    (School of Automotive Studies, Tongji University, Shanghai 201804, China
    Clean Energy Automotive Engineering Center, Tongji University, Shanghai 201804, China)

  • Haifeng Dai

    (School of Automotive Studies, Tongji University, Shanghai 201804, China
    Clean Energy Automotive Engineering Center, Tongji University, Shanghai 201804, China)

  • Fenglai Pei

    (Shanghai Motor Vehicle Inspection Certification & Tech Innovation Center Co., Ltd., Shanghai 201804, China)

  • Pingwen Ming

    (School of Automotive Studies, Tongji University, Shanghai 201804, China
    Clean Energy Automotive Engineering Center, Tongji University, Shanghai 201804, China)

  • Xuezhe Wei

    (School of Automotive Studies, Tongji University, Shanghai 201804, China
    Clean Energy Automotive Engineering Center, Tongji University, Shanghai 201804, China)

  • Jiangdong Zhou

    (Nantong Bing Energy Co., Ltd., Nantong 226500, China)

Abstract

Electrochemical impedance spectroscopy is one of the important tools for the performance analysis and diagnosis of proton exchange membrane fuel cells. The equivalent circuit model is an effective method for electrochemical impedance spectroscopy resolution. In this paper, four typical equivalent circuit models are selected to comprehensively compare and analyze the difference in the fitting results of the models for the electrochemical impedance spectroscopy under different working conditions (inlet pressure, stoichiometry, and humidity) from the perspective of the fitting accuracy, change trend of the model parameters, and the goodness of fit. The results show that the fitting accuracy of the model with the Warburg element is the best for all under each working condition. When considering the goodness of fit, the model with constant phase components is the best choice for fitting electrochemical impedance spectroscopy under different inlet pressure and air stoichiometry. However, under different air humidity, the model with the Warburg element is best. This work can help to promote the development of internal state analysis, estimation, and diagnosis of the fuel cell based on the equivalent circuit modeling of electrochemical impedance spectroscopy.

Suggested Citation

  • Lei Zhao & Haifeng Dai & Fenglai Pei & Pingwen Ming & Xuezhe Wei & Jiangdong Zhou, 2022. "A Comparative Study of Equivalent Circuit Models for Electro-Chemical Impedance Spectroscopy Analysis of Proton Exchange Membrane Fuel Cells," Energies, MDPI, vol. 15(1), pages 1-16, January.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:1:p:386-:d:718484
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    References listed on IDEAS

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    1. Zhou, Daming & Gao, Fei & Breaz, Elena & Ravey, Alexandre & Miraoui, Abdellatif, 2017. "Degradation prediction of PEM fuel cell using a moving window based hybrid prognostic approach," Energy, Elsevier, vol. 138(C), pages 1175-1186.
    2. Steven Chu & Arun Majumdar, 2012. "Opportunities and challenges for a sustainable energy future," Nature, Nature, vol. 488(7411), pages 294-303, August.
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    Cited by:

    1. Wang, Chuanjie & Li, Jia & Zhang, Siao & Li, Xiaoke & Duan, Xiao & Wu, Yongquan & Zhang, Qinghao & Yang, Tianrang & Liu, Jianguo, 2024. "High-precision identification of polarization processes of proton exchange membrane fuel cells through relaxation time analysis: Targeted experimental design and verification," Applied Energy, Elsevier, vol. 367(C).
    2. Andrea Baricci & Andrea Casalegno, 2023. "Experimental Analysis of Catalyst Layer Operation in a High-Temperature Proton Exchange Membrane Fuel Cell by Electrochemical Impedance Spectroscopy," Energies, MDPI, vol. 16(12), pages 1-17, June.

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