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Challenges and Perspectives for Doping Strategy for Manganese-Based Zinc-ion Battery Cathode

Author

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  • Bomian Zhang

    (State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China)

  • Jinghui Chen

    (State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China)

  • Weiyi Sun

    (State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China)

  • Yubo Shao

    (State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China)

  • Lei Zhang

    (State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, China
    Department of Physical Science and Technology, School of Science, Wuhan University of Technology, Wuhan 430070, China
    Hainan Institute, Wuhan University of Technology, Wuhan 430070, China)

  • Kangning Zhao

    (Laboratory of Advanced Separations, Ecole Polytechnique Federale de Lausanne, 1951 Sion, Switzerland)

Abstract

As one of the most appealing options for large-scale energy storage systems, the commercialization of aqueous zinc-ion batteries (AZIBs) has received considerable attention due to their cost effectiveness and inherent safety. A potential cathode material for the commercialization of AZIBs is the manganese-based cathode, but it suffers from poor cycle stability, owing to the Jahn–Teller effect, which leads to the dissolution of Mn in the electrolyte, as well as low electron/ion conductivity. In order to solve these problems, various strategies have been adopted to improve the stability of manganese-based cathode materials. Among those, the doping strategy has become popular, where the dopant is inserted into the intrinsic crystal structures of electrode materials, which would stabilize them and tune the electronic state of the redox center to realize high ion/electron transport. Herein, we summarize the ion doping strategy from the following aspects: (1) synthesis strategy of doped manganese-based oxides; (2) valence-dependent dopant ions in manganese-based oxides; (3) optimization mechanism of ion doping in zinc-manganese battery. Lastly, an in-depth understanding and future perspectives of ion doping strategy in electrode materials are provided for the commercialization of manganese-based zinc-ion batteries.

Suggested Citation

  • Bomian Zhang & Jinghui Chen & Weiyi Sun & Yubo Shao & Lei Zhang & Kangning Zhao, 2022. "Challenges and Perspectives for Doping Strategy for Manganese-Based Zinc-ion Battery Cathode," Energies, MDPI, vol. 15(13), pages 1-20, June.
    • Handle: RePEc:gam:jeners:v:15:y:2022:i:13:p:4698-:d:848667
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    1. Enze Hu & Huifang Li & Yizhou Zhang & Xiaojun Wang & Zhiming Liu, 2023. "Recent Progresses on Vanadium Sulfide Cathodes for Aqueous Zinc-Ion Batteries," Energies, MDPI, vol. 16(2), pages 1-18, January.
    2. Mikhail A. Kamenskii & Filipp S. Volkov & Svetlana N. Eliseeva & Elena G. Tolstopyatova & Veniamin V. Kondratiev, 2023. "Enhancement of Electrochemical Performance of Aqueous Zinc Ion Batteries by Structural and Interfacial Design of MnO 2 Cathodes: The Metal Ion Doping and Introduction of Conducting Polymers," Energies, MDPI, vol. 16(7), pages 1-44, April.

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