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Carbon-dioxide-to-methanol intensification with supersonic separators: Extra-carbonated natural gas purification via carbon capture and utilization

Author

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  • Arinelli, Lara de Oliveira
  • Brigagão, George Victor
  • Wiesberg, Igor Lapenda
  • Teixeira, Alexandre Mendonça
  • de Medeiros, José Luiz
  • Araújo, Ofélia de Queiroz F.

Abstract

A novel carbon-capture-and-utilization route from extra-carbonated natural gas using low-cost/low-carbon chloralkali hydrogen is disclosed. Methanol and methane-rich gas are produced without direct carbon emissions and also with low indirect emissions assuming the local electricity-matrix as 87% non-emitting. Carbon dioxide removed from raw natural gas via cryogenic extractive distillation with methanol entrainer, feeds a new Carbon-Dioxide-to-Methanol hydrogenation route intensified by supersonic separators with liquid water injection for greater methanol conversion per pass in the synthesis-loop and greater methanol recovery in the separation system. Intensified Carbon-Dioxide-to-Methanol is designed economically optimizing water/methanol injection-ratios and maximum Mach numbers of supersonic separators. Extra-carbonated natural gas processing coupled to intensified Carbon-Dioxide-to-Methanol is techno-economically assessed, demonstrating that supersonic intensification entails 2% greater methanol production, 11% less power consumption and 7.5% greater net value comparatively to non-intensified counterpart. The intensified process removes 99.2% of CO2 from extra-carbonated gas and was analyzed at two methanol scales [8021.5 t/d, 1692.3 t/d] giving, respectively, [9.5, 41.5] payback-years, and [2896.4MMUSD, 41.37MMUSD] net values (60years). A critical feasibility factor is low-cost/low-carbon by-product hydrogen from chloralkali industries, for which the break-even prices were respectively evaluated for the two scales as [685USD/tH2, 358USD/tH2]. A third, better and safer, option is to couple intensified Carbon-Dioxide-to-Methanol to large-scale Carbon-Dioxide-to-Enhanced-Oil-Recovery providing hedging against insufficient offer of low-cost/low-carbon hydrogen while practically keeping the project net value (60years) despite twofold investment.

Suggested Citation

  • Arinelli, Lara de Oliveira & Brigagão, George Victor & Wiesberg, Igor Lapenda & Teixeira, Alexandre Mendonça & de Medeiros, José Luiz & Araújo, Ofélia de Queiroz F., 2022. "Carbon-dioxide-to-methanol intensification with supersonic separators: Extra-carbonated natural gas purification via carbon capture and utilization," Renewable and Sustainable Energy Reviews, Elsevier, vol. 161(C).
    • Handle: RePEc:eee:rensus:v:161:y:2022:i:c:s1364032122003318
    DOI: 10.1016/j.rser.2022.112424
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    1. Wang, Shiwei & Wang, Chao & Ding, Hongbing & Li, Shujuan, 2024. "Evaluation of dynamic behaviors in varied swirling flows for high-pressure offshore natural gas supersonic dehydration," Energy, Elsevier, vol. 300(C).
    2. Wang, Shiwei & Wang, Chao & Ding, Hongbing & Zhang, Yu & Dong, Yuanyuan & Wen, Chuang, 2023. "Joule-Thomson effect and flow behavior for energy-efficient dehydration of high-pressure natural gas in supersonic separator," Energy, Elsevier, vol. 279(C).

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