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Experimental study on catalytic pyrolysis of rape straw with the active cathode material of spent lithium-ion batteries and HZSM-5 as the tandem catalysts

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  • Jiang, Jiaxin
  • Li, Xiaohua
  • Shao, Shanshan
  • Sun, Jiayuan
  • Yu, Zining
  • Cai, Yixi

Abstract

Effect of calcination temperature on the chemical composition, porous structure of cathode materials of spent lithium batteries (lithium iron phosphate, LFP; lithium nickel-cobalt manganate, NCM), and the production of high value-added products in the catalytic pyrolysis of rape straw with active cathode materials and HZSM-5 as the tandem catalysts were studied. The X-ray difraction and N2 adsorption-desorption analysis revealed that Fe2O3 and Co1.29Ni1.71O4 were mainly included in the LFP and NCM cathode materials calcined at 600 °C (LFP600 and NCM600), and the BET surface area of LFP600 and NCM600 reached the highest of 11.41 m2/g and 24.10 m2/g. In terms of catalytic performance, both LFP600 and NCM600 cathode materials showed best bond-breaking effect. Comparing these two cathode materials, LFP600 exhibited the better bond-breaking effect, while NCM600 presented a good deoxygenation effect. Finally, the synergistic effect of active cathode material and HZSM-5 was studied, and the quantitative yield of benzene, toluene and xylene reached 11.41 wt% and 10.96 wt% with the optimized calcined cathode material and HZSM-5 mass ratio of 1:5. In this study, it provides a new way to make high-valued utilization of solid wastes like agricultural and forest residues and spent lithium battery to produce clean and renewable energy.

Suggested Citation

  • Jiang, Jiaxin & Li, Xiaohua & Shao, Shanshan & Sun, Jiayuan & Yu, Zining & Cai, Yixi, 2023. "Experimental study on catalytic pyrolysis of rape straw with the active cathode material of spent lithium-ion batteries and HZSM-5 as the tandem catalysts," Renewable Energy, Elsevier, vol. 204(C), pages 803-811.
    • Handle: RePEc:eee:renene:v:204:y:2023:i:c:p:803-811
    DOI: 10.1016/j.renene.2022.12.102
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    References listed on IDEAS

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    1. Zeng, Jimin & Xiao, Rui & Zhang, Shuai & Zhang, Huiyan & Zeng, Dewang & Qiu, Yu & Ma, Zhong, 2018. "Identifying iron-based oxygen carrier reduction during biomass chemical looping gasification on a thermogravimetric fixed-bed reactor," Applied Energy, Elsevier, vol. 229(C), pages 404-412.
    2. Li, Xiangyu & Li, Guangyu & Li, Jian & Yu, Yanqing & Feng, Yu & Chen, Qun & Komarneni, Sridhar & Wang, Yujue, 2016. "Producing petrochemicals from catalytic fast pyrolysis of corn fermentation residual by-products generated from citric acid production," Renewable Energy, Elsevier, vol. 89(C), pages 331-338.
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    Cited by:

    1. Fan, Yongsheng & Yang, Jiaheng & Xu, Anjun & Zhu, Jinjiao & Shi, Yunxi, 2024. "Bio-aromatics synthesis via catalytic pyrolysis of cellulose with lithium-ion battery cathodes and modified HZSM-5 coupled in-situ plasma mode," Renewable Energy, Elsevier, vol. 226(C).

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