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Gold nanoparticles mixed multiwall carbon nanotubes, supported on graphene nano-ribbons (Au-NT-G) as an efficient reduction electrode for Polymer Electrolyte Membrane fuel cells (PEMFC)

Author

Listed:
  • Latif, Hamid
  • Wasif, Danish
  • Rasheed, Saba
  • Sattar, Abdul
  • Rafique, M. Shahid
  • Anwar, Abdul Waheed
  • Zaheer, S.
  • Shabbir, Syeda Ammara
  • Imtiaz, Ayesha
  • Qutab, Mehwish
  • Usman, Arslan

Abstract

This research reports fabrication of three Polymer Electrolyte Membrane fuel cells (PEMFC) using composite of gold nanoparticles and nanotube graphene by varying concentration of Gold nanoparticles. The outer most layer of multiwall carbon nanotubes is un-zipped and nano ribbons of graphene are developed to attain a durable electrode. Moreover, the addition of gold nanoparticles adds benefit of better conductance over usual platinum electrodes. The effect of changing gold concentration on properties of composite material as well as fuel cell performance is investigated. The presence of gold nanoparticles and graphene nano-ribbons attached to carbon nanotubes are identified using SEM, TEM, and Raman analysis. Cyclic voltammetry analysis has showed that increase in concentration of gold nano particles improves the performance of fuel cell. EIS analysis reveled that the polarization resistance decreased by increasing the Au concentration. Thermal Gravimetric Analysis proved the thermal stability of composite material. Maximum power density of 242.29 mWcm−2 is achieved for the highest concentration of Gold nanoparticles.

Suggested Citation

  • Latif, Hamid & Wasif, Danish & Rasheed, Saba & Sattar, Abdul & Rafique, M. Shahid & Anwar, Abdul Waheed & Zaheer, S. & Shabbir, Syeda Ammara & Imtiaz, Ayesha & Qutab, Mehwish & Usman, Arslan, 2020. "Gold nanoparticles mixed multiwall carbon nanotubes, supported on graphene nano-ribbons (Au-NT-G) as an efficient reduction electrode for Polymer Electrolyte Membrane fuel cells (PEMFC)," Renewable Energy, Elsevier, vol. 154(C), pages 767-773.
    • Handle: RePEc:eee:renene:v:154:y:2020:i:c:p:767-773
    DOI: 10.1016/j.renene.2020.03.061
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    References listed on IDEAS

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    1. Beltrán-Gastélum, M. & Salazar-Gastélum, M.I. & Félix-Navarro, R.M. & Pérez-Sicairos, S. & Reynoso-Soto, E.A. & Lin, S.W. & Flores-Hernández, J.R. & Romero-Castañón, T. & Albarrán-Sánchez, I.L. & Para, 2016. "Evaluation of PtAu/MWCNT (Multiwalled Carbon Nanotubes) electrocatalyst performance as cathode of a proton exchange membrane fuel cell," Energy, Elsevier, vol. 109(C), pages 446-455.
    2. Daud, W.R.W. & Rosli, R.E. & Majlan, E.H. & Hamid, S.A.A. & Mohamed, R. & Husaini, T., 2017. "PEM fuel cell system control: A review," Renewable Energy, Elsevier, vol. 113(C), pages 620-638.
    3. Nandan, Ravi & Goswami, Gopal Krishna & Nanda, Karuna Kar, 2017. "Direct synthesis of Pt-free catalyst on gas diffusion layer of fuel cell and usage of high boiling point fuels for efficient utilization of waste heat," Applied Energy, Elsevier, vol. 205(C), pages 1050-1058.
    4. Zhu, Jingyu & Tan, Jinzhu & Pan, Qing & Liu, Zenghui & Hou, Qiong, 2019. "Effects of Mg2+ contamination on the performance of proton exchange membrane fuel cell," Energy, Elsevier, vol. 189(C).
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    Cited by:

    1. Han, Yuan & Zhang, Houcheng, 2022. "Potentiality of elastocaloric cooling system for high-temperature proton exchange membrane fuel cell waste heat harvesting," Renewable Energy, Elsevier, vol. 200(C), pages 1166-1179.

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