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Experimental investigation on a novel phase change material composites coupled with graphite film used for thermal management of lithium-ion batteries

Author

Listed:
  • Luo, Xiaohang
  • Guo, Quangui
  • Li, Xiangfen
  • Tao, Zechao
  • Lei, Shiwen
  • Liu, Junqing
  • Kang, Libin
  • Zheng, Dongfang
  • Liu, Zhanjun

Abstract

Thermal management system is a key component to maintain the performance of lithium-ion batteries in electric vehicles. Cooling technology based on phase change materials with single-phase transition range has been proposed by many researchers but the temperature control of batteries is not ideal for high charge/discharge rates and cycle tests. Herein, we designed a novel phase change material consisting of paraffin with dual-phase transition ranges (around 34 °C and 48 °C), expanded graphite (thermal conductivity = 40 W/m K), and epoxy resin with a mass ratio of 5:2:3. This material was combined with graphite film (in-plane thermal conductivity of 1400 W/m K) to prepare a thermal management module. Graphite film and expanded graphite form an excellent heat conduction structure. Epoxy resin endows this composite with satisfactory mechanical properties, even at 70 °C. The paraffin provides a double buffer effect that minimizes the temperature increase of the batteries and the temperature differences between the batteries in the pack due to the broad phase transition range. As a result, the maximum temperature of the batteries is 33 °C and the maximum temperature difference between the batteries is only 1.4 °C, even at the highest 4C discharge rate. In addition, the maximum temperature of the batteries is only 44.8 °C after six extreme cycles.

Suggested Citation

  • Luo, Xiaohang & Guo, Quangui & Li, Xiangfen & Tao, Zechao & Lei, Shiwen & Liu, Junqing & Kang, Libin & Zheng, Dongfang & Liu, Zhanjun, 2020. "Experimental investigation on a novel phase change material composites coupled with graphite film used for thermal management of lithium-ion batteries," Renewable Energy, Elsevier, vol. 145(C), pages 2046-2055.
    • Handle: RePEc:eee:renene:v:145:y:2020:i:c:p:2046-2055
    DOI: 10.1016/j.renene.2019.07.112
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    Citations

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    Cited by:

    1. Weng, Jingwen & Xiao, Changren & Yang, Xiaoqing & Ouyang, Dongxu & Chen, Mingyi & Zhang, Guoqing & Lee Waiming, Eric & Kit Yuen, Richard Kwowk & Wang, Jian, 2022. "An energy-saving battery thermal management strategy coupling tubular phase-change-material with dynamic liquid cooling under different ambient temperatures," Renewable Energy, Elsevier, vol. 195(C), pages 918-930.
    2. Murali, G. & Sravya, G.S.N. & Jaya, J. & Naga Vamsi, V., 2021. "A review on hybrid thermal management of battery packs and it's cooling performance by enhanced PCM," Renewable and Sustainable Energy Reviews, Elsevier, vol. 150(C).
    3. Ma, Ying & Yang, Heng & Zuo, Hongyan & Zuo, Qingsong & He, Xiaoxiang & Chen, Wei & Wei, Rongrong, 2023. "EG@Bi-MOF derived porous carbon/lauric acid composite phase change materials for thermal management of batteries," Energy, Elsevier, vol. 272(C).
    4. Zhang, Jiangyun & Shao, Dan & Jiang, Liqin & Zhang, Guoqing & Wu, Hongwei & Day, Rodney & Jiang, Wenzhao, 2022. "Advanced thermal management system driven by phase change materials for power lithium-ion batteries: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 159(C).
    5. Shen, Zu-Guo & Chen, Shuai & Liu, Xun & Chen, Ben, 2021. "A review on thermal management performance enhancement of phase change materials for vehicle lithium-ion batteries," Renewable and Sustainable Energy Reviews, Elsevier, vol. 148(C).
    6. Yi, Feng & E, Jiaqiang & Zhang, Bin & Zuo, Hongyan & Wei, Kexiang & Chen, Jingwei & Zhu, Hong & Zhu, Hao & Deng, Yuanwang, 2022. "Effects analysis on heat dissipation characteristics of lithium-ion battery thermal management system under the synergism of phase change material and liquid cooling method," Renewable Energy, Elsevier, vol. 181(C), pages 472-489.
    7. Weng, Jingwen & Xiao, Changren & Ouyang, Dongxu & Yang, Xiaoqing & Chen, Mingyi & Zhang, Guoqing & Yuen, Richard Kwok Kit & Wang, Jian, 2022. "Mitigation effects on thermal runaway propagation of structure-enhanced phase change material modules with flame retardant additives," Energy, Elsevier, vol. 239(PC).
    8. Chen, Mingyi & Yu, Yue & Ouyang, Dongxu & Weng, Jingwen & Zhao, Luyao & Wang, Jian & Chen, Yin, 2024. "Research progress of enhancing battery safety with phase change materials," Renewable and Sustainable Energy Reviews, Elsevier, vol. 189(PA).
    9. Zhao, Yanqi & Zou, Boyang & Zhang, Tongtong & Jiang, Zhu & Ding, Jianning & Ding, Yulong, 2022. "A comprehensive review of composite phase change material based thermal management system for lithium-ion batteries," Renewable and Sustainable Energy Reviews, Elsevier, vol. 167(C).
    10. Liang, Jialin & Gan, Yunhua & Tan, Meixian & Li, Yong, 2020. "Multilayer electrochemical-thermal coupled modeling of unbalanced discharging in a serially connected lithium-ion battery module," Energy, Elsevier, vol. 209(C).

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