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Numerical studies of the influences of bypass on hydrogen separation in a multichannel Pd membrane system

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  • Chen, Wei-Hsin
  • Tsai, Ching-Wei
  • Lin, Yu-Li

Abstract

A multichannel palladium (Pd) membrane system in association with flow bypass is designed for hydrogen separation with high recovery, and the mass transfer phenomena in the system are simulated by developing a computational fluid dynamics (CFD) model. Two Pd membranes are installed in the system. The predictions suggest that the H2 recovery (HR) can be substantially improved by the bypass. The higher the feed gas Reynolds number, the more pronounced the improvement of H2 recovery by the bypass. The HR by the first membrane is independent of the bypass ratio (BR), revealing that the enhancement of HR is completely contributed by the second membrane. An increase in H2/CO2 molar ratio in the feed gas reduces HR, but raises the H2 permeation rate. The maximum HR by the second membrane always develops at the feed gas Reynolds number (Rer,M1) of 500, regardless of bypass ratio. This reveals that the aforementioned Reynolds number is an appropriate condition for H2 separation in the designed membrane system. Based on the HR in the absence of flow bypass (i.e., BR = 0), the higher the Rer,M1, the larger the intensification of H2 permeation. A contour map and a correlation from regression analysis in terms of Rer,M1 and BR are established. Under a desired H2 recovery, the combination of Rer,M1 and BR can be suggested to provide flexible operation for H2 separation in the membrane system.

Suggested Citation

  • Chen, Wei-Hsin & Tsai, Ching-Wei & Lin, Yu-Li, 2017. "Numerical studies of the influences of bypass on hydrogen separation in a multichannel Pd membrane system," Renewable Energy, Elsevier, vol. 104(C), pages 259-270.
    • Handle: RePEc:eee:renene:v:104:y:2017:i:c:p:259-270
    DOI: 10.1016/j.renene.2016.12.032
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    References listed on IDEAS

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    1. Chen, Wei-Hsin & Hsia, Ming-Hsien & Chi, Yen-Hsun & Lin, Yu-Li & Yang, Chang-Chung, 2014. "Polarization phenomena of hydrogen-rich gas in high-permeance Pd and Pd–Cu membrane tubes," Applied Energy, Elsevier, vol. 113(C), pages 41-50.
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    4. Chen, Wei-Hsin & Lin, Shih-Cheng, 2015. "Reaction phenomena of catalytic partial oxidation of methane under the impact of carbon dioxide addition and heat recirculation," Energy, Elsevier, vol. 82(C), pages 206-217.
    5. Barbir, Frano, 2009. "Transition to renewable energy systems with hydrogen as an energy carrier," Energy, Elsevier, vol. 34(3), pages 308-312.
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    1. Chen, Wei-Hsin & Li, Shu-Cheng & Lim, Steven & Chen, Zih-Yu & Juan, Joon Ching, 2021. "Reaction and hydrogen production phenomena of ethanol steam reforming in a catalytic membrane reactor," Energy, Elsevier, vol. 220(C).
    2. Chen, Wei-Hsin & Kuo, Pei-Chi & Lin, Yu-Li, 2019. "Evolutionary computation for maximizing CO2 and H2 separation in multiple-tube palladium-membrane systems," Applied Energy, Elsevier, vol. 235(C), pages 299-310.

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