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Growth patterns in electrodeposition

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  • Léger, Christophe
  • Servant, Laurent
  • Bruneel, Jean Luc
  • Argoul, Françoise

Abstract

In that short review of growth processes in electrodeposition, we aim at discussing the relevant physical and chemical mechanisms which are likely to influence the dynamics of these growth processes and the morphology of the electrodeposits obtained in thin gap geometries. Electrodeposition has been early recognized as a paradigm experiment for reproducing diffusiondashlimited aggregation (DLA) morphologies as produced by the model of Witten and Sanders. The obvious similitude between DLA clusters and thin gap electrodeposits for some parameter values opened some fundamental issues about the correspondence of these experimental systems with DLA processes. We want to address in this paper the greater complexity of an electrodeposition process, in particular as far as the interfacial chemical and electrochemical kinetics is concerned. Our discussion is illustrated by an experimental analysis of copper electrodeposition in thin gap cells, based on interferometric, spectroscopic and optical inspection of both the deposit morphology and its composition and of the concentration fields around the deposit. Supported by these experimental investigations of copper electrodeposition in thin gap cells, we show that chemistry based argumentations are unescapable to explain the observed dynamical processes.

Suggested Citation

  • Léger, Christophe & Servant, Laurent & Bruneel, Jean Luc & Argoul, Françoise, 1999. "Growth patterns in electrodeposition," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 263(1), pages 305-314.
    • Handle: RePEc:eee:phsmap:v:263:y:1999:i:1:p:305-314
    DOI: 10.1016/S0378-4371(98)00484-1
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    1. Blanche, S. & Mayaux, M.-J. & Veber, F. & Landreau, A. & Courpotin, C. & Vilmer, E. & Ciraru-Vigneron, N. & Floch, C. & Tricoire, J. & Noseda, G. & Jean-Marc, J. & Rouzioux, C., 1996. "Separation between HIV-positive women and their children: The French prospective study, 1986 through 1993," American Journal of Public Health, American Public Health Association, vol. 86(3), pages 376-381.
    2. Argoul, F. & Kuhn, A., 1995. "The influence of transport and reaction processes on the morphology of a metal electrodeposit in thin gap geometry," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 213(1), pages 209-231.
    3. Julio Berbel & Julio Gallego & Horacio Sagues, 1991. "Marketing goals vs. business profitability: An interactive multiple criteria decision-making approach," Agribusiness, John Wiley & Sons, Ltd., vol. 7(6), pages 537-549.
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    Cited by:

    1. Aarão Reis, F.D.A., 2005. "Statistical models of diffusion and aggregation for coke formation in a catalyst pore," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 350(2), pages 407-417.

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