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Identifying degradation mechanisms in lithium-ion batteries with coating defects at the cathode

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  • David, Lamuel
  • Ruther, Rose E.
  • Mohanty, Debasish
  • Meyer, Harry M.
  • Sheng, Yangping
  • Kalnaus, Sergiy
  • Daniel, Claus
  • Wood, David L.

Abstract

Understanding the effect of electrode manufacturing defects on lithium-ion battery (LIB) performance is key to reducing the scrap rate and cost during cell manufacturing. In this regard, it is necessary to quantify the impact of various defects that are generated during the electrode coating process. To this end, we have tested large-format 0.5 Ah LiNi0.5Mn0.3Co0.2O2/graphite pouch cells with defects intentionally introduced into the cathode coating. Different types of coating defects were tested including agglomerates, pinholes, and non-uniform coating. Electrodes with larger non-coated surface had greater capacity fade than baseline electrodes, while pinholes and agglomerates did not affect performance adversely. Post cycle analysis of electrodes showed that the anode facing the defective region in the cathode was clearly impacted by the defect. Further characterization using Raman spectroscopy, X-ray photoelectron spectroscopy, and X-ray diffraction provided evidence for a proposed mechanism for material degradation related to the most detrimental type of coating defect.

Suggested Citation

  • David, Lamuel & Ruther, Rose E. & Mohanty, Debasish & Meyer, Harry M. & Sheng, Yangping & Kalnaus, Sergiy & Daniel, Claus & Wood, David L., 2018. "Identifying degradation mechanisms in lithium-ion batteries with coating defects at the cathode," Applied Energy, Elsevier, vol. 231(C), pages 446-455.
    • Handle: RePEc:eee:appene:v:231:y:2018:i:c:p:446-455
    DOI: 10.1016/j.apenergy.2018.09.073
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    References listed on IDEAS

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    Cited by:

    1. Daniel Evans & Paul-Martin Luc & Claas Tebruegge & Julia Kowal, 2023. "Detection of Manufacturing Defects in Lithium-Ion Batteries-Analysis of the Potential of Computed Tomography Imaging," Energies, MDPI, vol. 16(19), pages 1-17, October.
    2. Yang, Yang & Yuan, Wei & Zhang, Xiaoqing & Ke, Yuzhi & Qiu, Zhiqiang & Luo, Jian & Tang, Yong & Wang, Chun & Yuan, Yuhang & Huang, Yao, 2020. "A review on structuralized current collectors for high-performance lithium-ion battery anodes," Applied Energy, Elsevier, vol. 276(C).
    3. Pan, Yue & Kong, Xiangdong & Yuan, Yuebo & Sun, Yukun & Han, Xuebing & Yang, Hongxin & Zhang, Jianbiao & Liu, Xiaoan & Gao, Panlong & Li, Yihui & Lu, Languang & Ouyang, Minggao, 2023. "Detecting the foreign matter defect in lithium-ion batteries based on battery pilot manufacturing line data analyses," Energy, Elsevier, vol. 262(PB).
    4. Yuan, Yuebo & Wang, Hewu & Han, Xuebing & Pan, Yue & Sun, Yukun & Kong, Xiangdong & Lu, Languang & Ouyang, Minggao, 2024. "The local lithium plating caused by anode crack defect in Li-ion battery," Applied Energy, Elsevier, vol. 361(C).

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