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Numerical and experimental investigation of pollutant formation and emissions in a full-scale cylindrical heating unit of a condensing gas boiler

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  • Hinrichs, Jörn
  • Felsmann, Daniel
  • Schweitzer-De Bortoli, Stefan
  • Tomczak, Heinz-Jörg
  • Pitsch, Heinz

Abstract

The condensing gas boiler technology has received increasing attention due to its very high efficiency of more than 90%, which is an increase of more than 15% compared to non-condensing boiler devices. With this, condensing gas boilers offer the chance to decrease the energy consumption and CO2 emissions for domestic hot water and heating. While further increasing the energy efficiency of condensing boiler devices, pollutant emissions have to be considered as well since they are a threat to human health and therefore subject to continuously intensified governmental restrictions. In this study, a comprehensive investigation of the full-scale heating unit of a commercial condensing gas boiler was performed. Local measurements at different axial positions revealed an inhomogeneous distribution of CO and NO emissions due to varying temperature levels in the burnt region. Resolved simulations with finite rate chemistry identified a quenching of the CO oxidation reactions due to a fast depletion of OH radicals. Consequently, the CO concentration in the cooled exhaust gas is significantly higher than expected from chemical equilibrium calculations. Regarding NO formation, the majority of NO is found to be produced within the flame front, while only a small part is formed in the postflame region. A detailed pathway analysis pointed out that besides the well known thermal NO pathway, the NNH pathway has the highest contribution to the overall NO emissions. These insights open up possibilities to develop new condensing boiler generations where emission levels below the permitted limits can be achieved.

Suggested Citation

  • Hinrichs, Jörn & Felsmann, Daniel & Schweitzer-De Bortoli, Stefan & Tomczak, Heinz-Jörg & Pitsch, Heinz, 2018. "Numerical and experimental investigation of pollutant formation and emissions in a full-scale cylindrical heating unit of a condensing gas boiler," Applied Energy, Elsevier, vol. 229(C), pages 977-989.
    • Handle: RePEc:eee:appene:v:229:y:2018:i:c:p:977-989
    DOI: 10.1016/j.apenergy.2018.08.011
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    1. McKenna, R.C. & Bchini, Q. & Weinand, J.M. & Michaelis, J. & König, S. & Köppel, W. & Fichtner, W., 2018. "The future role of Power-to-Gas in the energy transition: Regional and local techno-economic analyses in Baden-Württemberg," Applied Energy, Elsevier, vol. 212(C), pages 386-400.
    2. Johnson, Geoffrey & Beausoleil-Morrison, Ian, 2016. "The calibration and validation of a model for predicting the performance of gas-fired tankless water heaters in domestic hot water applications," Applied Energy, Elsevier, vol. 177(C), pages 740-750.
    3. Weber, C & Gebhardt, B & Fahl, U, 2002. "Market transformation for energy efficient technologies — success factors and empirical evidence for gas condensing boilers," Energy, Elsevier, vol. 27(3), pages 287-315.
    4. Lee, Seungro & Kum, Sung-Min & Lee, Chang-Eon, 2011. "An experimental study of a cylindrical multi-hole premixed burner for the development of a condensing gas boiler," Energy, Elsevier, vol. 36(7), pages 4150-4157.
    5. Mujeebu, M. Abdul & Abdullah, M.Z. & Bakar, M.Z. Abu & Mohamad, A.A. & Abdullah, M.K., 2009. "Applications of porous media combustion technology - A review," Applied Energy, Elsevier, vol. 86(9), pages 1365-1375, September.
    6. Shang, Sheng & Li, Xianting & Chen, Wei & Wang, Baolong & Shi, Wenxing, 2017. "A total heat recovery system between the flue gas and oxidizing air of a gas-fired boiler using a non-contact total heat exchanger," Applied Energy, Elsevier, vol. 207(C), pages 613-623.
    7. Badr, O. & Probert, S. D., 1993. "Oxides of nitrogen in the Earth's atmosphere: Trends, sources, sinks and environmental impacts," Applied Energy, Elsevier, vol. 46(1), pages 1-67.
    8. Badr, O. & Probert, S. D., 1995. "Sinks and environmental impacts for atmospheric carbon monoxide," Applied Energy, Elsevier, vol. 50(4), pages 339-372.
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    Cited by:

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    3. Lamioni, Rachele & Bronzoni, Cristiana & Folli, Marco & Tognotti, Leonardo & Galletti, Chiara, 2022. "Feeding H2-admixtures to domestic condensing boilers: Numerical simulations of combustion and pollutant formation in multi-hole burners," Applied Energy, Elsevier, vol. 309(C).
    4. Liu, Fengguo & Zheng, Longfeng & Zhang, Rui, 2020. "Emissions and thermal efficiency for premixed burners in a condensing gas boiler," Energy, Elsevier, vol. 202(C).
    5. Yılmaz, Semih & Kumlutaş, Dilek & Yücekaya, Utku Alp & Cumbul, Ahmet Yakup, 2021. "Prediction of the equilibrium compositions in the combustion products of a domestic boiler," Energy, Elsevier, vol. 233(C).
    6. Ahmadi, Ziaulhaq & Zabetian Targhi, Mohammad, 2021. "Thermal performance investigation of a premixed surface flame burner used in the domestic heating boilers," Energy, Elsevier, vol. 236(C).
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