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The enhanced enzymatic performance of carbonic anhydrase on the reaction rate between CO2 and aqueous solutions of sterically hindered amines

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  • Neslisah Cihan
  • Ozge Yuksel Orhan

Abstract

The kinetics of the reactions of carbon dioxide (CO2) with aqueous solutions of two different sterically hindered amines (SHAs), 2‐amino‐2‐ethyl‐1,3‐propanediol (AEPD) and 2‐amino‐2‐methyl‐1,3‐propanediol (AMPD), in the presence and absence of carbonic anhydrase (CA) was investigated experimentally using stopped‐flow conductimetry. The amine concentration, CA concentration, and temperature were varied within the ranges of 0.1–0.5 kmol·m–3, 0–125 g·m–3, and 298–353 K, respectively. Based on pseudo first‐order reaction conditions, the intrinsic reaction rate (ko) was obtained according to a modified termolecular reaction mechanism. The obtained results showed that the reaction rate between the SHA solutions (either aqueous AEPD or aqueous AMPD) and CO2 was enhanced significantly upon adding small amounts of CA as a promoter. Such a result supports the use of the aforementioned solvent system as a candidate for CO2 capture. © 2020 Society of Chemical Industry and John Wiley & Sons, Ltd.

Suggested Citation

  • Neslisah Cihan & Ozge Yuksel Orhan, 2020. "The enhanced enzymatic performance of carbonic anhydrase on the reaction rate between CO2 and aqueous solutions of sterically hindered amines," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 10(5), pages 925-937, October.
    • Handle: RePEc:wly:greenh:v:10:y:2020:i:5:p:925-937
    DOI: 10.1002/ghg.2012
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    1. Zhang, Zhien & Pan, Shu-Yuan & Li, Hao & Cai, Jianchao & Olabi, Abdul Ghani & Anthony, Edward John & Manovic, Vasilije, 2020. "Recent advances in carbon dioxide utilization," Renewable and Sustainable Energy Reviews, Elsevier, vol. 125(C).
    2. Pal, Animesh & Uddin, Kutub & Saha, Bidyut Baran & Thu, Kyaw & Kil, Hyun-Sig & Yoon, Seong-Ho & Miyawaki, Jin, 2020. "A benchmark for CO2 uptake onto newly synthesized biomass-derived activated carbons," Applied Energy, Elsevier, vol. 264(C).
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