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Scaling of the strange-metal scattering in unconventional superconductors

Author

Listed:
  • Jie Yuan

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Qihong Chen

    (Chinese Academy of Sciences
    Songshan Lake Materials Laboratory)

  • Kun Jiang

    (Chinese Academy of Sciences)

  • Zhongpei Feng

    (Chinese Academy of Sciences
    Songshan Lake Materials Laboratory)

  • Zefeng Lin

    (Chinese Academy of Sciences)

  • Heshan Yu

    (Chinese Academy of Sciences)

  • Ge He

    (Chinese Academy of Sciences)

  • Jinsong Zhang

    (Chinese Academy of Sciences)

  • Xingyu Jiang

    (Chinese Academy of Sciences)

  • Xu Zhang

    (Chinese Academy of Sciences)

  • Yujun Shi

    (Chinese Academy of Sciences)

  • Yanmin Zhang

    (Chinese Academy of Sciences)

  • Mingyang Qin

    (Chinese Academy of Sciences)

  • Zhi Gang Cheng

    (Chinese Academy of Sciences
    Songshan Lake Materials Laboratory)

  • Nobumichi Tamura

    (Advanced Light Source, Lawrence Berkeley National Laboratory)

  • Yi-feng Yang

    (Chinese Academy of Sciences)

  • Tao Xiang

    (Chinese Academy of Sciences
    Beijing Academy of Quantum Information Sciences)

  • Jiangping Hu

    (Chinese Academy of Sciences
    Songshan Lake Materials Laboratory)

  • Ichiro Takeuchi

    (University of Maryland
    University of Maryland)

  • Kui Jin

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences
    Songshan Lake Materials Laboratory)

  • Zhongxian Zhao

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences
    Songshan Lake Materials Laboratory)

Abstract

Marked evolution of properties with minute changes in the doping level is a hallmark of the complex chemistry that governs copper oxide superconductivity as manifested in the celebrated superconducting domes and quantum criticality taking place at precise compositions1–4. The strange-metal state, in which the resistivity varies linearly with temperature, has emerged as a central feature in the normal state of copper oxide superconductors5–9. The ubiquity of this behaviour signals an intimate link between the scattering mechanism and superconductivity10–12. However, a clear quantitative picture of the correlation has been lacking. Here we report the observation of precise quantitative scaling laws among the superconducting transition temperature (Tc), the linear-in-T scattering coefficient (A1) and the doping level (x) in electron-doped copper oxide La2–xCexCuO4 (LCCO). High-resolution characterization of epitaxial composition-spread films, which encompass the entire overdoped range of LCCO, has enabled us to systematically map its structural and transport properties with unprecedented accuracy and with increments of Δx = 0.0015. We have uncovered the relations Tc ~ (xc – x)0.5 ~ (A1□)0.5, where xc is the critical doping in which superconductivity disappears and A1□ is the coefficient of the linear resistivity per CuO2 plane. The striking similarity of the Tc versus A1□ relation among copper oxides, iron-based and organic superconductors may be an indication of a common mechanism of the strange-metal behaviour and unconventional superconductivity in these systems.

Suggested Citation

  • Jie Yuan & Qihong Chen & Kun Jiang & Zhongpei Feng & Zefeng Lin & Heshan Yu & Ge He & Jinsong Zhang & Xingyu Jiang & Xu Zhang & Yujun Shi & Yanmin Zhang & Mingyang Qin & Zhi Gang Cheng & Nobumichi Tam, 2022. "Scaling of the strange-metal scattering in unconventional superconductors," Nature, Nature, vol. 602(7897), pages 431-436, February.
  • Handle: RePEc:nat:nature:v:602:y:2022:i:7897:d:10.1038_s41586-021-04305-5
    DOI: 10.1038/s41586-021-04305-5
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    Cited by:

    1. J. Ayres & M. Berben & C. Duffy & R. D. H. Hinlopen & Y.-T. Hsu & A. Cuoghi & M. Leroux & I. Gilmutdinov & M. Massoudzadegan & D. Vignolles & Y. Huang & T. Kondo & T. Takeuchi & S. Friedemann & A. Car, 2024. "Universal correlation between H-linear magnetoresistance and T-linear resistivity in high-temperature superconductors," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    2. Shu Cai & Jinyu Zhao & Ni Ni & Jing Guo & Run Yang & Pengyu Wang & Jinyu Han & Sijin Long & Yazhou Zhou & Qi Wu & Xianggang Qiu & Tao Xiang & Robert J. Cava & Liling Sun, 2023. "The breakdown of both strange metal and superconducting states at a pressure-induced quantum critical point in iron-pnictide superconductors," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    3. Matthew Brahlek & Joseph D. Roth & Lei Zhang & Megan Briggeman & Patrick Irvin & Jason Lapano & Jeremy Levy & Turan Birol & Roman Engel-Herbert, 2024. "Hidden transport phenomena in an ultraclean correlated metal," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

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