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Continuous Mott transition in semiconductor moiré superlattices

Author

Listed:
  • Tingxin Li

    (Cornell University)

  • Shengwei Jiang

    (Cornell University)

  • Lizhong Li

    (Cornell University)

  • Yang Zhang

    (Massachusetts Institute of Technology)

  • Kaifei Kang

    (Cornell University)

  • Jiacheng Zhu

    (Cornell University)

  • Kenji Watanabe

    (National Institute for Materials Science)

  • Takashi Taniguchi

    (National Institute for Materials Science)

  • Debanjan Chowdhury

    (Cornell University)

  • Liang Fu

    (Massachusetts Institute of Technology)

  • Jie Shan

    (Cornell University
    Cornell University
    Kavli Institute at Cornell for Nanoscale Science)

  • Kin Fai Mak

    (Cornell University
    Cornell University
    Kavli Institute at Cornell for Nanoscale Science)

Abstract

The evolution of a Landau Fermi liquid into a non-magnetic Mott insulator with increasing electronic interactions is one of the most puzzling quantum phase transitions in physics1–6. The vicinity of the transition is believed to host exotic states of matter such as quantum spin liquids4–7, exciton condensates8 and unconventional superconductivity1. Semiconductor moiré materials realize a highly controllable Hubbard model simulator on a triangular lattice9–22, providing a unique opportunity to drive a metal–insulator transition (MIT) via continuous tuning of the electronic interactions. Here, by electrically tuning the effective interaction strength in MoTe2/WSe2 moiré superlattices, we observe a continuous MIT at a fixed filling of one electron per unit cell. The existence of quantum criticality is supported by the scaling collapse of the resistance, a continuously vanishing charge gap as the critical point is approached from the insulating side, and a diverging quasiparticle effective mass from the metallic side. We also observe a smooth evolution of the magnetic susceptibility across the MIT and no evidence of long-range magnetic order down to ~5% of the Curie–Weiss temperature. This signals an abundance of low-energy spinful excitations on the insulating side that is further corroborated by the Pomeranchuk effect observed on the metallic side. Our results are consistent with the universal critical theory of a continuous Mott transition in two dimensions4,23.

Suggested Citation

  • Tingxin Li & Shengwei Jiang & Lizhong Li & Yang Zhang & Kaifei Kang & Jiacheng Zhu & Kenji Watanabe & Takashi Taniguchi & Debanjan Chowdhury & Liang Fu & Jie Shan & Kin Fai Mak, 2021. "Continuous Mott transition in semiconductor moiré superlattices," Nature, Nature, vol. 597(7876), pages 350-354, September.
  • Handle: RePEc:nat:nature:v:597:y:2021:i:7876:d:10.1038_s41586-021-03853-0
    DOI: 10.1038/s41586-021-03853-0
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    Citations

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    Cited by:

    1. Wai-Ga D. Ho & Peng Zhang & Kristjan Haule & Jennifer M. Jackson & Vladimir Dobrosavljević & Vasilije V. Dobrosavljevic, 2024. "Quantum critical phase of FeO spans conditions of Earth’s lower mantle," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. Binjie Zheng & Junzhuan Wang & Qianghua Wang & Xin Su & Tianye Huang & Songlin Li & Fengqiu Wang & Yi Shi & Xiaomu Wang, 2022. "Quantum criticality of excitonic Mott metal-insulator transitions in black phosphorus," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    3. Beini Gao & Daniel G. Suárez-Forero & Supratik Sarkar & Tsung-Sheng Huang & Deric Session & Mahmoud Jalali Mehrabad & Ruihao Ni & Ming Xie & Pranshoo Upadhyay & Jonathan Vannucci & Sunil Mittal & Kenj, 2024. "Excitonic Mott insulator in a Bose-Fermi-Hubbard system of moiré WS2/WSe2 heterobilayer," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    4. Yuting Tan & Pak Ki Henry Tsang & Vladimir Dobrosavljević, 2022. "Disorder-dominated quantum criticality in moiré bilayers," Nature Communications, Nature, vol. 13(1), pages 1-6, December.
    5. David Barcons Ruiz & Hanan Herzig Sheinfux & Rebecca Hoffmann & Iacopo Torre & Hitesh Agarwal & Roshan Krishna Kumar & Lorenzo Vistoli & Takashi Taniguchi & Kenji Watanabe & Adrian Bachtold & Frank H., 2022. "Engineering high quality graphene superlattices via ion milled ultra-thin etching masks," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    6. Yanhao Tang & Jie Gu & Song Liu & Kenji Watanabe & Takashi Taniguchi & James C. Hone & Kin Fai Mak & Jie Shan, 2022. "Dielectric catastrophe at the Wigner-Mott transition in a moiré superlattice," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    7. Zeya Li & Junwei Huang & Ling Zhou & Zian Xu & Feng Qin & Peng Chen & Xiaojun Sun & Gan Liu & Chengqi Sui & Caiyu Qiu & Yangfan Lu & Huiyang Gou & Xiaoxiang Xi & Toshiya Ideue & Peizhe Tang & Yoshihir, 2023. "An anisotropic van der Waals dielectric for symmetry engineering in functionalized heterointerfaces," Nature Communications, Nature, vol. 14(1), pages 1-9, December.

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