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Correlation-driven topological phases in magic-angle twisted bilayer graphene

Author

Listed:
  • Youngjoon Choi

    (T. J. Watson Laboratory of Applied Physics, California Institute of Technology
    Institute for Quantum Information and Matter, California Institute of Technology
    California Institute of Technology)

  • Hyunjin Kim

    (T. J. Watson Laboratory of Applied Physics, California Institute of Technology
    Institute for Quantum Information and Matter, California Institute of Technology
    California Institute of Technology)

  • Yang Peng

    (California State University)

  • Alex Thomson

    (Institute for Quantum Information and Matter, California Institute of Technology
    California Institute of Technology
    California Institute of Technology)

  • Cyprian Lewandowski

    (Institute for Quantum Information and Matter, California Institute of Technology
    California Institute of Technology
    California Institute of Technology)

  • Robert Polski

    (T. J. Watson Laboratory of Applied Physics, California Institute of Technology
    Institute for Quantum Information and Matter, California Institute of Technology)

  • Yiran Zhang

    (T. J. Watson Laboratory of Applied Physics, California Institute of Technology
    Institute for Quantum Information and Matter, California Institute of Technology
    California Institute of Technology)

  • Harpreet Singh Arora

    (T. J. Watson Laboratory of Applied Physics, California Institute of Technology
    Institute for Quantum Information and Matter, California Institute of Technology)

  • Kenji Watanabe

    (National Institute for Materials Science)

  • Takashi Taniguchi

    (National Institute for Materials Science)

  • Jason Alicea

    (Institute for Quantum Information and Matter, California Institute of Technology
    California Institute of Technology
    California Institute of Technology)

  • Stevan Nadj-Perge

    (T. J. Watson Laboratory of Applied Physics, California Institute of Technology
    Institute for Quantum Information and Matter, California Institute of Technology)

Abstract

Magic-angle twisted bilayer graphene (MATBG) exhibits a range of correlated phenomena that originate from strong electron–electron interactions. These interactions make the Fermi surface highly susceptible to reconstruction when ±1, ±2 and ±3 electrons occupy each moiré unit cell, and lead to the formation of various correlated phases1–4. Although some phases have been shown to have a non-zero Chern number5,6, the local microscopic properties and topological character of many other phases have not yet been determined. Here we introduce a set of techniques that use scanning tunnelling microscopy to map the topological phases that emerge in MATBG in a finite magnetic field. By following the evolution of the local density of states at the Fermi level with electrostatic doping and magnetic field, we create a local Landau fan diagram that enables us to assign Chern numbers directly to all observed phases. We uncover the existence of six topological phases that arise from integer fillings in finite fields and that originate from a cascade of symmetry-breaking transitions driven by correlations7,8. These topological phases can form only for a small range of twist angles around the magic angle, which further differentiates them from the Landau levels observed near charge neutrality. Moreover, we observe that even the charge-neutrality Landau spectrum taken at low fields is considerably modified by interactions, exhibits prominent electron–hole asymmetry, and features an unexpectedly large splitting between zero Landau levels (about 3 to 5 millielectronvolts). Our results show how strong electronic interactions affect the MATBG band structure and lead to correlation-enabled topological phases.

Suggested Citation

  • Youngjoon Choi & Hyunjin Kim & Yang Peng & Alex Thomson & Cyprian Lewandowski & Robert Polski & Yiran Zhang & Harpreet Singh Arora & Kenji Watanabe & Takashi Taniguchi & Jason Alicea & Stevan Nadj-Per, 2021. "Correlation-driven topological phases in magic-angle twisted bilayer graphene," Nature, Nature, vol. 589(7843), pages 536-541, January.
  • Handle: RePEc:nat:nature:v:589:y:2021:i:7843:d:10.1038_s41586-020-03159-7
    DOI: 10.1038/s41586-020-03159-7
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    Citations

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    Cited by:

    1. Sami Dzsaber & Diego A. Zocco & Alix McCollam & Franziska Weickert & Ross McDonald & Mathieu Taupin & Gaku Eguchi & Xinlin Yan & Andrey Prokofiev & Lucas M. K. Tang & Bryan Vlaar & Laurel E. Winter & , 2022. "Control of electronic topology in a strongly correlated electron system," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    2. Yuting Tan & Pak Ki Henry Tsang & Vladimir Dobrosavljević, 2022. "Disorder-dominated quantum criticality in moiré bilayers," Nature Communications, Nature, vol. 13(1), pages 1-6, December.
    3. Saisab Bhowmik & Bhaskar Ghawri & Youngju Park & Dongkyu Lee & Suvronil Datta & Radhika Soni & K. Watanabe & T. Taniguchi & Arindam Ghosh & Jeil Jung & U. Chandni, 2023. "Spin-orbit coupling-enhanced valley ordering of malleable bands in twisted bilayer graphene on WSe2," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    4. Canxun Zhang & Tiancong Zhu & Tomohiro Soejima & Salman Kahn & Kenji Watanabe & Takashi Taniguchi & Alex Zettl & Feng Wang & Michael P. Zaletel & Michael F. Crommie, 2023. "Local spectroscopy of a gate-switchable moiré quantum anomalous Hall insulator," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    5. Pratap Chandra Adak & Subhajit Sinha & Debasmita Giri & Dibya Kanti Mukherjee & Chandan & L. D. Varma Sangani & Surat Layek & Ayshi Mukherjee & Kenji Watanabe & Takashi Taniguchi & H. A. Fertig & Arij, 2022. "Perpendicular electric field drives Chern transitions and layer polarization changes in Hofstadter bands," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    6. Anushree Datta & M. J. Calderón & A. Camjayi & E. Bascones, 2023. "Heavy quasiparticles and cascades without symmetry breaking in twisted bilayer graphene," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    7. Le Liu & Shihao Zhang & Yanbang Chu & Cheng Shen & Yuan Huang & Yalong Yuan & Jinpeng Tian & Jian Tang & Yiru Ji & Rong Yang & Kenji Watanabe & Takashi Taniguchi & Dongxia Shi & Jianpeng Liu & Wei Yan, 2022. "Isospin competitions and valley polarized correlated insulators in twisted double bilayer graphene," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    8. Daniel Shaffer & Jian Wang & Luiz H. Santos, 2022. "Unconventional self-similar Hofstadter superconductivity from repulsive interactions," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    9. Si-yu Li & Zhengwen Wang & Yucheng Xue & Yingbo Wang & Shihao Zhang & Jianpeng Liu & Zheng Zhu & Kenji Watanabe & Takashi Taniguchi & Hong-jun Gao & Yuhang Jiang & Jinhai Mao, 2022. "Imaging topological and correlated insulating states in twisted monolayer-bilayer graphene," Nature Communications, Nature, vol. 13(1), pages 1-7, December.

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