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Strange-metal behaviour in a pure ferromagnetic Kondo lattice

Author

Listed:
  • Bin Shen

    (Zhejiang University)

  • Yongjun Zhang

    (Zhejiang University)

  • Yashar Komijani

    (Rutgers University)

  • Michael Nicklas

    (Max Planck Institute for Chemical Physics of Solids)

  • Robert Borth

    (Max Planck Institute for Chemical Physics of Solids)

  • An Wang

    (Zhejiang University)

  • Ye Chen

    (Zhejiang University)

  • Zhiyong Nie

    (Zhejiang University)

  • Rui Li

    (Zhejiang University)

  • Xin Lu

    (Zhejiang University)

  • Hanoh Lee

    (Zhejiang University
    Sungkyunkwan University)

  • Michael Smidman

    (Zhejiang University)

  • Frank Steglich

    (Zhejiang University
    Max Planck Institute for Chemical Physics of Solids)

  • Piers Coleman

    (Rutgers University
    University of London)

  • Huiqiu Yuan

    (Zhejiang University
    Nanjing University)

Abstract

A wide range of metals exhibit anomalous electrical and thermodynamic properties when tuned to a quantum critical point (QCP), although the origins of such strange metals have posed a long-standing mystery. The frequent association of strange metals with unconventional superconductivity and antiferromagnetic QCPs1–4 has led to the belief that they are highly entangled quantum states5. By contrast, ferromagnets are regarded as an unlikely setting for strange metals, because they are weakly entangled and their QCPs are often interrupted by competing phases or first-order phase transitions6–8. Here we provide evidence that the pure ferromagnetic Kondo lattice9,10 CeRh6Ge4 becomes a strange metal at a pressure-induced QCP. Measurements of the specific heat and resistivity under pressure demonstrate that the ferromagnetic transition is continuously suppressed to zero temperature, revealing a strange-metal behaviour around the QCP. We argue that strong magnetic anisotropy has a key role in this process, injecting entanglement in the form of triplet resonating valence bonds into the ordered ferromagnet. We show that a singular transformation in the patterns of the entanglement between local moments and conduction electrons, from triplet resonating valence bonds to Kondo-entangled singlet pairs at the QCP, causes a jump in the Fermi surface volume—a key driver of strange-metallic behaviour. Our results open up a direction for research into ferromagnetic quantum criticality and establish an alternative setting for the strange-metal phenomenon. Most importantly, strange-metal behaviour at a ferromagnetic QCP suggests that quantum entanglement—not the destruction of antiferromagnetism—is the common driver of the varied behaviours of strange metals.

Suggested Citation

  • Bin Shen & Yongjun Zhang & Yashar Komijani & Michael Nicklas & Robert Borth & An Wang & Ye Chen & Zhiyong Nie & Rui Li & Xin Lu & Hanoh Lee & Michael Smidman & Frank Steglich & Piers Coleman & Huiqiu , 2020. "Strange-metal behaviour in a pure ferromagnetic Kondo lattice," Nature, Nature, vol. 579(7797), pages 51-55, March.
  • Handle: RePEc:nat:nature:v:579:y:2020:i:7797:d:10.1038_s41586-020-2052-z
    DOI: 10.1038/s41586-020-2052-z
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    Cited by:

    1. Subhasis Samanta & Hwiwoo Park & Chanhyeon Lee & Sungmin Jeon & Hengbo Cui & Yong-Xin Yao & Jungseek Hwang & Kwang-Yong Choi & Heung-Sik Kim, 2024. "Emergence of flat bands and ferromagnetic fluctuations via orbital-selective electron correlations in Mn-based kagome metal," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    2. Zhen-Yu Liu & Heng Jin & Yao Zhang & Kai Fan & Ting-Fei Guo & Hao-Jun Qin & Lan-Fang Zhu & Lian-Zhi Yang & Wen-Hao Zhang & Bing Huang & Ying-Shuang Fu, 2024. "Charge-density wave mediated quasi-one-dimensional Kondo lattice in stripe-phase monolayer 1T-NbSe2," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

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