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Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet

Author

Listed:
  • Jia-Xin Yin

    (Princeton University)

  • Songtian S. Zhang

    (Princeton University)

  • Hang Li

    (Institute of Physics, Chinese Academy of Sciences)

  • Kun Jiang

    (Boston College)

  • Guoqing Chang

    (Princeton University)

  • Bingjing Zhang

    (Renmin University of China)

  • Biao Lian

    (Princeton University)

  • Cheng Xiang

    (Peking University
    University of Chinese Academy of Sciences)

  • Ilya Belopolski

    (Princeton University)

  • Hao Zheng

    (Princeton University)

  • Tyler A. Cochran

    (Princeton University)

  • Su-Yang Xu

    (Princeton University)

  • Guang Bian

    (Princeton University)

  • Kai Liu

    (Renmin University of China)

  • Tay-Rong Chang

    (National Cheng Kung University)

  • Hsin Lin

    (Institute of Physics, Academia Sinica)

  • Zhong-Yi Lu

    (Renmin University of China)

  • Ziqiang Wang

    (Boston College)

  • Shuang Jia

    (Peking University
    University of Chinese Academy of Sciences)

  • Wenhong Wang

    (Institute of Physics, Chinese Academy of Sciences)

  • M. Zahid Hasan

    (Princeton University
    Lawrence Berkeley National Laboratory)

Abstract

Owing to the unusual geometry of kagome lattices—lattices made of corner-sharing triangles—their electrons are useful for studying the physics of frustrated, correlated and topological quantum electronic states1–9. In the presence of strong spin–orbit coupling, the magnetic and electronic structures of kagome lattices are further entangled, which can lead to hitherto unknown spin–orbit phenomena. Here we use a combination of vector-magnetic-field capability and scanning tunnelling microscopy to elucidate the spin–orbit nature of the kagome ferromagnet Fe3Sn2 and explore the associated exotic correlated phenomena. We discover that a many-body electronic state from the kagome lattice couples strongly to the vector field with three-dimensional anisotropy, exhibiting a magnetization-driven giant nematic (two-fold-symmetric) energy shift. Probing the fermionic quasi-particle interference reveals consistent spontaneous nematicity—a clear indication of electron correlation—and vector magnetization is capable of altering this state, thus controlling the many-body electronic symmetry. These spin-driven giant electronic responses go well beyond Zeeman physics and point to the realization of an underlying correlated magnetic topological phase. The tunability of this kagome magnet reveals a strong interplay between an externally applied field, electronic excitations and nematicity, providing new ways of controlling spin–orbit properties and exploring emergent phenomena in topological or quantum materials10–12.

Suggested Citation

  • Jia-Xin Yin & Songtian S. Zhang & Hang Li & Kun Jiang & Guoqing Chang & Bingjing Zhang & Biao Lian & Cheng Xiang & Ilya Belopolski & Hao Zheng & Tyler A. Cochran & Su-Yang Xu & Guang Bian & Kai Liu & , 2018. "Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet," Nature, Nature, vol. 562(7725), pages 91-95, October.
  • Handle: RePEc:nat:nature:v:562:y:2018:i:7725:d:10.1038_s41586-018-0502-7
    DOI: 10.1038/s41586-018-0502-7
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    Citations

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    Cited by:

    1. Xitong Xu & Jia-Xin Yin & Wenlong Ma & Hung-Ju Tien & Xiao-Bin Qiang & P. V. Sreenivasa Reddy & Huibin Zhou & Jie Shen & Hai-Zhou Lu & Tay-Rong Chang & Zhe Qu & Shuang Jia, 2022. "Topological charge-entropy scaling in kagome Chern magnet TbMn6Sn6," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    2. Heda Zhang & Jahyun Koo & Chunqiang Xu & Milos Sretenovic & Binghai Yan & Xianglin Ke, 2022. "Exchange-biased topological transverse thermoelectric effects in a Kagome ferrimagnet," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    3. Subhasis Samanta & Hwiwoo Park & Chanhyeon Lee & Sungmin Jeon & Hengbo Cui & Yong-Xin Yao & Jungseek Hwang & Kwang-Yong Choi & Heung-Sik Kim, 2024. "Emergence of flat bands and ferromagnetic fluctuations via orbital-selective electron correlations in Mn-based kagome metal," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    4. Ruiqing Cheng & Lei Yin & Yao Wen & Baoxing Zhai & Yuzheng Guo & Zhaofu Zhang & Weitu Liao & Wenqi Xiong & Hao Wang & Shengjun Yuan & Jian Jiang & Chuansheng Liu & Jun He, 2022. "Ultrathin ferrite nanosheets for room-temperature two-dimensional magnetic semiconductors," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    5. J. N. Graham & C. Mielke III & D. Das & T. Morresi & V. Sazgari & A. Suter & T. Prokscha & H. Deng & R. Khasanov & S. D. Wilson & A. C. Salinas & M. M. Martins & Y. Zhong & K. Okazaki & Z. Wang & M. Z, 2024. "Depth-dependent study of time-reversal symmetry-breaking in the kagome superconductor AV3Sb5," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    6. Sen Zhou & Ziqiang Wang, 2022. "Chern Fermi pocket, topological pair density wave, and charge-4e and charge-6e superconductivity in kagomé superconductors," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    7. Hangyu Zhou & Manuel dos Santos Dias & Youguang Zhang & Weisheng Zhao & Samir Lounis, 2024. "Kagomerization of transition metal monolayers induced by two-dimensional hexagonal boron nitride," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    8. Han Wu & Lei Chen & Paul Malinowski & Bo Gyu Jang & Qinwen Deng & Kirsty Scott & Jianwei Huang & Jacob P. C. Ruff & Yu He & Xiang Chen & Chaowei Hu & Ziqin Yue & Ji Seop Oh & Xiaokun Teng & Yucheng Gu, 2024. "Reversible non-volatile electronic switching in a near-room-temperature van der Waals ferromagnet," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    9. Wenliang Zhang & Teguh Citra Asmara & Yi Tseng & Junbo Li & Yimin Xiong & Yuan Wei & Tianlun Yu & Carlos William Galdino & Zhijia Zhang & Kurt Kummer & Vladimir N. Strocov & Y. Soh & Thorsten Schmitt , 2024. "Spin waves and orbital contribution to ferromagnetism in a topological metal," Nature Communications, Nature, vol. 15(1), pages 1-9, December.

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