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Mapping molecular motions leading to charge delocalization with ultrabright electrons

Author

Listed:
  • Meng Gao

    (University of Toronto
    University of Hamburg, Hamburg Center for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany)

  • Cheng Lu

    (University of Toronto)

  • Hubert Jean-Ruel

    (University of Toronto
    University of Hamburg, Hamburg Center for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany)

  • Lai Chung Liu

    (University of Toronto
    University of Hamburg, Hamburg Center for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany)

  • Alexander Marx

    (University of Hamburg, Hamburg Center for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany)

  • Ken Onda

    (Interactive Research Center of Science, Tokyo Institute of Technology, Nagatsuta, Midori-ku, Yokohama 226-8502, Japan
    PRESTO, Japan Science and Technology Agency)

  • Shin-ya Koshihara

    (Tokyo Institute of Technology, Ōokayama, Meguro-ku, Tokyo 152-8551, Japan
    CREST, Japan Science and Technology Agency (JST), 5-3, Yonbancho, Chiyoda-ku, Tokyo 102-8666, Japan)

  • Yoshiaki Nakano

    (Research Center for Low Temperature and Materials Sciences, Kyoto University)

  • Xiangfeng Shao

    (Research Center for Low Temperature and Materials Sciences, Kyoto University
    Present address: State Key Laboratory of Applied Organic Chemistry, Lanzhou University, 222 Tianshui South Road, Lanzhou 730000, Gansu, China.)

  • Takaaki Hiramatsu

    (Faculty of Agriculture, Meijo University)

  • Gunzi Saito

    (Faculty of Agriculture, Meijo University)

  • Hideki Yamochi

    (Research Center for Low Temperature and Materials Sciences, Kyoto University)

  • Ryan R. Cooney

    (University of Toronto
    University of Hamburg, Hamburg Center for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany)

  • Gustavo Moriena

    (University of Toronto
    University of Hamburg, Hamburg Center for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany)

  • Germán Sciaini

    (University of Toronto
    University of Hamburg, Hamburg Center for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany)

  • R. J. Dwayne Miller

    (University of Toronto
    University of Hamburg, Hamburg Center for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg, Germany)

Abstract

An ultrabright femtosecond electron source is used to monitor the molecular motions in the organic salt (EDO-TTF)2PF6 as it undergoes its photo-induced insulator-to-metal phase transition.

Suggested Citation

  • Meng Gao & Cheng Lu & Hubert Jean-Ruel & Lai Chung Liu & Alexander Marx & Ken Onda & Shin-ya Koshihara & Yoshiaki Nakano & Xiangfeng Shao & Takaaki Hiramatsu & Gunzi Saito & Hideki Yamochi & Ryan R. C, 2013. "Mapping molecular motions leading to charge delocalization with ultrabright electrons," Nature, Nature, vol. 496(7445), pages 343-346, April.
    • Handle: RePEc:nat:nature:v:496:y:2013:i:7445:d:10.1038_nature12044
    DOI: 10.1038/nature12044
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    Cited by:

    1. Marius Hervé & Gaël Privault & Elzbieta Trzop & Shintaro Akagi & Yves Watier & Serhane Zerdane & Ievgeniia Chaban & Ricardo G. Torres Ramírez & Celine Mariette & Alix Volte & Marco Cammarata & Matteo , 2024. "Ultrafast and persistent photoinduced phase transition at room temperature monitored by streaming powder diffraction," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    2. Yuri Saida & Thomas Gauthier & Hiroo Suzuki & Satoshi Ohmura & Ryo Shikata & Yui Iwasaki & Godai Noyama & Misaki Kishibuchi & Yuichiro Tanaka & Wataru Yajima & Nicolas Godin & Gaël Privault & Tomoharu, 2024. "Photoinduced dynamics during electronic transfer from narrow to wide bandgap layers in one-dimensional heterostructured materials," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    3. Le Zeng & Tiexin Zhang & Renhai Liu & Wenming Tian & Kaifeng Wu & Jingyi Zhu & Zhonghe Wang & Cheng He & Jing Feng & Xiangyang Guo & Abdoulkader Ibro Douka & Chunying Duan, 2023. "Chalcogen-bridged coordination polymer for the photocatalytic activation of aryl halides," Nature Communications, Nature, vol. 14(1), pages 1-13, December.
    4. Yifeng Jiang & Stuart Hayes & Simon Bittmann & Antoine Sarracini & Lai Chung Liu & Henrike M. Müller-Werkmeister & Atsuhiro Miyawaki & Masaki Hada & Shinnosuke Nakano & Ryoya Takahashi & Samiran Banu , 2024. "Direct observation of photoinduced sequential spin transition in a halogen-bonded hybrid system by complementary ultrafast optical and electron probes," Nature Communications, Nature, vol. 15(1), pages 1-10, December.

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