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Visualizing heavy fermions emerging in a quantum critical Kondo lattice

Author

Listed:
  • Pegor Aynajian

    (Princeton University)

  • Eduardo H. da Silva Neto

    (Princeton University)

  • András Gyenis

    (Princeton University)

  • Ryan E. Baumbach

    (Los Alamos National Laboratory)

  • J. D. Thompson

    (Los Alamos National Laboratory)

  • Zachary Fisk

    (University of California)

  • Eric D. Bauer

    (Los Alamos National Laboratory)

  • Ali Yazdani

    (Princeton University)

Abstract

In solids containing elements with f orbitals, the interaction between f-electron spins and those of itinerant electrons leads to the development of low-energy fermionic excitations with a heavy effective mass. These excitations are fundamental to the appearance of unconventional superconductivity and non-Fermi-liquid behaviour observed in actinide- and lanthanide-based compounds. Here we use spectroscopic mapping with the scanning tunnelling microscope to detect the emergence of heavy excitations with lowering of temperature in a prototypical family of cerium-based heavy-fermion compounds. We demonstrate the sensitivity of the tunnelling process to the composite nature of these heavy quasiparticles, which arises from quantum entanglement of itinerant conduction and f electrons. Scattering and interference of the composite quasiparticles is used to resolve their energy–momentum structure and to extract their mass enhancement, which develops with decreasing temperature. The lifetime of the emergent heavy quasiparticles reveals signatures of enhanced scattering and their spectral lineshape shows evidence of energy–temperature scaling. These findings demonstrate that proximity to a quantum critical point results in critical damping of the emergent heavy excitation of our Kondo lattice system.

Suggested Citation

  • Pegor Aynajian & Eduardo H. da Silva Neto & András Gyenis & Ryan E. Baumbach & J. D. Thompson & Zachary Fisk & Eric D. Bauer & Ali Yazdani, 2012. "Visualizing heavy fermions emerging in a quantum critical Kondo lattice," Nature, Nature, vol. 486(7402), pages 201-206, June.
  • Handle: RePEc:nat:nature:v:486:y:2012:i:7402:d:10.1038_nature11204
    DOI: 10.1038/nature11204
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    Cited by:

    1. Kai Fan & Heng Jin & Bing Huang & Guijing Duan & Rong Yu & Zhen-Yu Liu & Hui-Nan Xia & Li-Si Liu & Yao Zhang & Tao Xie & Qiao-Yin Tang & Gang Chen & Wen-Hao Zhang & F. C. Chen & X. Luo & W. J. Lu & Y., 2024. "Artificial superconducting Kondo lattice in a van der Waals heterostructure," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    2. M. C. Rahn & K. Kummer & A. Hariki & K.-H. Ahn & J. Kuneš & A. Amorese & J. D. Denlinger & D.-H. Lu & M. Hashimoto & E. Rienks & M. Valvidares & F. Haslbeck & D. D. Byler & K. J. McClellan & E. D. Bau, 2022. "Kondo quasiparticle dynamics observed by resonant inelastic x-ray scattering," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    3. Wen Wan & Rishav Harsh & Antonella Meninno & Paul Dreher & Sandra Sajan & Haojie Guo & Ion Errea & Fernando Juan & Miguel M. Ugeda, 2023. "Evidence for ground state coherence in a two-dimensional Kondo lattice," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

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