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Nanomechanical oscillations in a single-C60 transistor

Author

Listed:
  • Hongkun Park

    (Department of Chemistry and
    Materials Sciences Division, Lawrence Berkeley National Laboratory
    Harvard University)

  • Jiwoong Park

    (University of California at Berkeley)

  • Andrew K. L. Lim

    (Department of Chemistry and)

  • Erik H. Anderson

    (Materials Sciences Division, Lawrence Berkeley National Laboratory)

  • A. Paul Alivisatos

    (Department of Chemistry and
    Materials Sciences Division, Lawrence Berkeley National Laboratory)

  • Paul L. McEuen

    (University of California at Berkeley
    Materials Sciences Division, Lawrence Berkeley National Laboratory)

Abstract

The motion of electrons through quantum dots is strongly modified by single-electron charging and the quantization of energy levels1,2. Much effort has been directed towards extending studies of electron transport to chemical nanostructures, including molecules3,4,5,6,7,8, nanocrystals9,10,11,12,13 and nanotubes14,15,16,17. Here we report the fabrication of single-molecule transistors based on individual C60 molecules connected to gold electrodes. We perform transport measurements that provide evidence for a coupling between the centre-of-mass motion of the C60 molecules and single-electron hopping18—a conduction mechanism that has not been observed previously in quantum dot studies. The coupling is manifest as quantized nano-mechanical oscillations of the C60 molecule against the gold surface, with a frequency of about 1.2 THz. This value is in good agreement with a simple theoretical estimate based on van der Waals and electrostatic interactions between C60 molecules and gold electrodes.

Suggested Citation

  • Hongkun Park & Jiwoong Park & Andrew K. L. Lim & Erik H. Anderson & A. Paul Alivisatos & Paul L. McEuen, 2000. "Nanomechanical oscillations in a single-C60 transistor," Nature, Nature, vol. 407(6800), pages 57-60, September.
    • Handle: RePEc:nat:nature:v:407:y:2000:i:6800:d:10.1038_35024031
    DOI: 10.1038/35024031
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    Cited by:

    1. Linan Meng & Na Xin & Chen Hu & Hassan Al Sabea & Miao Zhang & Hongyu Jiang & Yiru Ji & Chuancheng Jia & Zhuang Yan & Qinghua Zhang & Lin Gu & Xiaoyan He & Pramila Selvanathan & Lucie Norel & Stéphane, 2022. "Dual-gated single-molecule field-effect transistors beyond Moore’s law," Nature Communications, Nature, vol. 13(1), pages 1-6, December.
    2. Thanh Luan Phan & Sohyeon Seo & Yunhee Cho & Quoc An Vu & Young Hee Lee & Dinh Loc Duong & Hyoyoung Lee & Woo Jong Yu, 2022. "CNT-molecule-CNT (1D-0D-1D) van der Waals integration ferroelectric memory with 1-nm2 junction area," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    3. Lei Zhang & Chen Yang & Chenxi Lu & Xingxing Li & Yilin Guo & Jianning Zhang & Jinglong Lin & Zhizhou Li & Chuancheng Jia & Jinlong Yang & K. N. Houk & Fanyang Mo & Xuefeng Guo, 2022. "Precise electrical gating of the single-molecule Mizoroki-Heck reaction," Nature Communications, Nature, vol. 13(1), pages 1-11, December.

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