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Interplay between temperature and bandgap energies on the outdoor performance of perovskite/silicon tandem solar cells

Author

Listed:
  • Erkan Aydin

    (King Abdullah University of Science and Technology (KAUST))

  • Thomas G. Allen

    (King Abdullah University of Science and Technology (KAUST))

  • Michele De Bastiani

    (King Abdullah University of Science and Technology (KAUST))

  • Lujia Xu

    (King Abdullah University of Science and Technology (KAUST))

  • Jorge Ávila

    (King Abdullah University of Science and Technology (KAUST)
    Universidad de Valencia)

  • Michael Salvador

    (King Abdullah University of Science and Technology (KAUST))

  • Emmanuel Van Kerschaver

    (King Abdullah University of Science and Technology (KAUST))

  • Stefaan De Wolf

    (King Abdullah University of Science and Technology (KAUST))

Abstract

Perovskite/silicon tandem solar cells promise power conversion efficiencies beyond the Shockley–Queisser limit of single-junction devices; however, their actual outdoor performance is yet to be investigated. Here we fabricate 25% efficient two-terminal monolithic perovskite/silicon tandem solar cells and test them outdoors in a hot and sunny climate. We find that the temperature dependence of both the silicon and perovskite bandgaps—which follow opposing trends—shifts the devices away from current matching for two-terminal tandems that are optimized at standard test conditions. Consequently, we argue that the optimal perovskite bandgap energy at standard test conditions is

Suggested Citation

  • Erkan Aydin & Thomas G. Allen & Michele De Bastiani & Lujia Xu & Jorge Ávila & Michael Salvador & Emmanuel Van Kerschaver & Stefaan De Wolf, 2020. "Interplay between temperature and bandgap energies on the outdoor performance of perovskite/silicon tandem solar cells," Nature Energy, Nature, vol. 5(11), pages 851-859, November.
    • Handle: RePEc:nat:natene:v:5:y:2020:i:11:d:10.1038_s41560-020-00687-4
    DOI: 10.1038/s41560-020-00687-4
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    Cited by:

    1. Ahmed A. Said & Erkan Aydin & Esma Ugur & Zhaojian Xu & Caner Deger & Badri Vishal & Aleš Vlk & Pia Dally & Bumin K. Yildirim & Randi Azmi & Jiang Liu & Edward A. Jackson & Holly M. Johnson & Manting , 2024. "Sublimed C60 for efficient and repeatable perovskite-based solar cells," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    2. Costas Prouskas & Angelos Mourkas & Georgios Zois & Elefterios Lidorikis & Panos Patsalas, 2022. "A New Type of Architecture of Dye-Sensitized Solar Cells as an Alternative Pathway to Outdoor Photovoltaics," Energies, MDPI, vol. 15(7), pages 1-14, March.
    3. Khan, Firoz & Rezgui, Béchir Dridi & Khan, Mohd Taukeer & Al-Sulaiman, Fahad, 2022. "Perovskite-based tandem solar cells: Device architecture, stability, and economic perspectives," Renewable and Sustainable Energy Reviews, Elsevier, vol. 165(C).
    4. Bahram Abdollahi Nejand & David B. Ritzer & Hang Hu & Fabian Schackmar & Somayeh Moghadamzadeh & Thomas Feeney & Roja Singh & Felix Laufer & Raphael Schmager & Raheleh Azmi & Milian Kaiser & Tobias Ab, 2022. "Scalable two-terminal all-perovskite tandem solar modules with a 19.1% efficiency," Nature Energy, Nature, vol. 7(7), pages 620-630, July.
    5. Fangyuan Ye & Shuo Zhang & Jonathan Warby & Jiawei Wu & Emilio Gutierrez-Partida & Felix Lang & Sahil Shah & Elifnaz Saglamkaya & Bowen Sun & Fengshuo Zu & Safa Shoaee & Haifeng Wang & Burkhard Stille, 2022. "Overcoming C60-induced interfacial recombination in inverted perovskite solar cells by electron-transporting carborane," Nature Communications, Nature, vol. 13(1), pages 1-12, December.

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