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Single crystal hybrid perovskite field-effect transistors

Author

Listed:
  • Weili Yu

    (King Abdullah University of Science and Technology (KAUST)
    Chinese Academy of Sciences (CAS))

  • Feng Li

    (King Abdullah University of Science and Technology (KAUST))

  • Liyang Yu

    (King Abdullah University of Science and Technology (KAUST))

  • Muhammad R. Niazi

    (King Abdullah University of Science and Technology (KAUST))

  • Yuting Zou

    (Chinese Academy of Sciences (CAS))

  • Daniel Corzo

    (King Abdullah University of Science and Technology (KAUST))

  • Aniruddha Basu

    (King Abdullah University of Science and Technology (KAUST))

  • Chun Ma

    (King Abdullah University of Science and Technology (KAUST))

  • Sukumar Dey

    (King Abdullah University of Science and Technology (KAUST))

  • Max L. Tietze

    (King Abdullah University of Science and Technology (KAUST)
    KU Leuven — University of Leuven)

  • Ulrich Buttner

    (King Abdullah University of Science and Technology (KAUST))

  • Xianbin Wang

    (King Abdullah University of Science and Technology (KAUST))

  • Zhihong Wang

    (King Abdullah University of Science and Technology (KAUST))

  • Mohamed N. Hedhili

    (King Abdullah University of Science and Technology (KAUST))

  • Chunlei Guo

    (Chinese Academy of Sciences (CAS)
    University of Rochester)

  • Tom Wu

    (King Abdullah University of Science and Technology (KAUST)
    University of New South Wales (UNSW))

  • Aram Amassian

    (King Abdullah University of Science and Technology (KAUST)
    North Carolina State University)

Abstract

The fields of photovoltaics, photodetection and light emission have seen tremendous activity in recent years with the advent of hybrid organic-inorganic perovskites. Yet, there have been far fewer reports of perovskite-based field-effect transistors. The lateral and interfacial transport requirements of transistors make them particularly vulnerable to surface contamination and defects rife in polycrystalline films and bulk single crystals. Here, we demonstrate a spatially-confined inverse temperature crystallization strategy which synthesizes micrometre-thin single crystals of methylammonium lead halide perovskites MAPbX3 (X = Cl, Br, I) with sub-nanometer surface roughness and very low surface contamination. These benefit the integration of MAPbX3 crystals into ambipolar transistors and yield record, room-temperature field-effect mobility up to 4.7 and 1.5 cm2 V−1 s−1 in p and n channel devices respectively, with 104 to 105 on-off ratio and low turn-on voltages. This work paves the way for integrating hybrid perovskite crystals into printed, flexible and transparent electronics.

Suggested Citation

  • Weili Yu & Feng Li & Liyang Yu & Muhammad R. Niazi & Yuting Zou & Daniel Corzo & Aniruddha Basu & Chun Ma & Sukumar Dey & Max L. Tietze & Ulrich Buttner & Xianbin Wang & Zhihong Wang & Mohamed N. Hedh, 2018. "Single crystal hybrid perovskite field-effect transistors," Nature Communications, Nature, vol. 9(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:9:y:2018:i:1:d:10.1038_s41467-018-07706-9
    DOI: 10.1038/s41467-018-07706-9
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    Cited by:

    1. Hyunho Lee & Hyung‐Jun Song, 2021. "Current status and perspective of colored photovoltaic modules," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 10(6), November.
    2. Huihui Zhu & Ao Liu & Kyu In Shim & Haksoon Jung & Taoyu Zou & Youjin Reo & Hyunjun Kim & Jeong Woo Han & Yimu Chen & Hye Yong Chu & Jun Hyung Lim & Hyung-Jun Kim & Sai Bai & Yong-Young Noh, 2022. "High-performance hysteresis-free perovskite transistors through anion engineering," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    3. Yao Ma & Leting Shan & Yiran Ying & Liang Shen & Yufeng Fu & Linfeng Fei & Yusheng Lei & Nailin Yue & Wei Zhang & Hong Zhang & Haitao Huang & Kai Yao & Junhao Chu, 2024. "Day-Night imaging without Infrared Cutfilter removal based on metal-gradient perovskite single crystal photodetector," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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