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Multifunctional nanocomposite hollow fiber membranes by solvent transfer induced phase separation

Author

Listed:
  • Martin F. Haase

    (Rowan University, Henry M. Rowan College of Engineering)

  • Harim Jeon

    (Department of Chemical and Biomolecular Engineering, University of Pennsylvania
    Department of Chemical and Biomolecular Engineering, Yonsei University)

  • Noah Hough

    (Rowan University, Henry M. Rowan College of Engineering)

  • Jong Hak Kim

    (Department of Chemical and Biomolecular Engineering, Yonsei University)

  • Kathleen J. Stebe

    (Department of Chemical and Biomolecular Engineering, University of Pennsylvania)

  • Daeyeon Lee

    (Department of Chemical and Biomolecular Engineering, University of Pennsylvania)

Abstract

The decoration of porous membranes with a dense layer of nanoparticles imparts useful functionality and can enhance membrane separation and anti-fouling properties. However, manufacturing of nanoparticle-coated membranes requires multiple steps and tedious processing. Here, we introduce a facile single-step method in which bicontinuous interfacially jammed emulsions are used to form nanoparticle-functionalized hollow fiber membranes. The resulting nanocomposite membranes prepared via solvent transfer-induced phase separation and photopolymerization have exceptionally high nanoparticle loadings (up to 50 wt% silica nanoparticles) and feature densely packed nanoparticles uniformly distributed over the entire membrane surfaces. These structurally well-defined, asymmetric membranes facilitate control over membrane flux and selectivity, enable the formation of stimuli responsive hydrogel nanocomposite membranes, and can be easily modified to introduce antifouling features. This approach forms a foundation for the formation of advanced nanocomposite membranes comprising diverse building blocks with potential applications in water treatment, industrial separations and as catalytic membrane reactors.

Suggested Citation

  • Martin F. Haase & Harim Jeon & Noah Hough & Jong Hak Kim & Kathleen J. Stebe & Daeyeon Lee, 2017. "Multifunctional nanocomposite hollow fiber membranes by solvent transfer induced phase separation," Nature Communications, Nature, vol. 8(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:8:y:2017:i:1:d:10.1038_s41467-017-01409-3
    DOI: 10.1038/s41467-017-01409-3
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    Cited by:

    1. Renita, A. Annam & Lakshmi, D. Shanthana & Maheswari, P. & Saxena, Mayank & Kumar, J. Aravind & Vigneswaran, V.S., 2024. "Energy recovery and clean water remediation using antibiofouling polysaccharide coated PAN hollow fiber membrane obtained via green route synthesis," Energy, Elsevier, vol. 294(C).
    2. Parisa Bazazi & Howard A. Stone & S. Hossein Hejazi, 2022. "Spongy all-in-liquid materials by in-situ formation of emulsions at oil-water interfaces," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    3. Chen, Xiaoqing & Ali, Imdad & Song, Lijian & Song, Peng & Zhang, Youchen & Maria, Semeniuk & Nazmus, Saadat & Yang, Weimin & Dhakal, Hom Nath & Li, Haoyi & Sain, Mohini & Ramakrishna, Seeram, 2020. "A review on recent advancement of nano-structured-fiber-based metal-air batteries and future perspective," Renewable and Sustainable Energy Reviews, Elsevier, vol. 134(C).

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