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Understanding materials challenges for rechargeable ion batteries with in situ transmission electron microscopy

Author

Listed:
  • Yifei Yuan

    (Argonne National Laboratory
    University of Illinois at Chicago)

  • Khalil Amine

    (Argonne National Laboratory)

  • Jun Lu

    (Argonne National Laboratory)

  • Reza Shahbazian-Yassar

    (University of Illinois at Chicago)

Abstract

An in-depth understanding of material behaviours under complex electrochemical environment is critical for the development of advanced materials for the next-generation rechargeable ion batteries. The dynamic conditions inside a working battery had not been intensively explored until the advent of various in situ characterization techniques. Real-time transmission electron microscopy of electrochemical reactions is one of the most significant breakthroughs poised to enable radical shift in our knowledge on how materials behave in the electrochemical environment. This review, therefore, summarizes the scientific discoveries enabled by in situ transmission electron microscopy, and specifically emphasizes the applicability of this technique to address the critical challenges in the rechargeable ion battery electrodes, electrolyte and their interfaces. New electrochemical systems such as lithium–oxygen, lithium–sulfur and sodium ion batteries are included, considering the rapidly increasing application of in situ transmission electron microscopy in these areas. A systematic comparison between lithium ion-based electrochemistry and sodium ion-based electrochemistry is also given in terms of their thermodynamic and kinetic differences. The effect of the electron beam on the validity of in situ observation is also covered. This review concludes by providing a renewed perspective for the future directions of in situ transmission electron microscopy in rechargeable ion batteries.

Suggested Citation

  • Yifei Yuan & Khalil Amine & Jun Lu & Reza Shahbazian-Yassar, 2017. "Understanding materials challenges for rechargeable ion batteries with in situ transmission electron microscopy," Nature Communications, Nature, vol. 8(1), pages 1-14, August.
    • Handle: RePEc:nat:natcom:v:8:y:2017:i:1:d:10.1038_ncomms15806
    DOI: 10.1038/ncomms15806
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    Cited by:

    1. Che Lah, Nurul Akmal, 2021. "Late transition metal nanocomplexes: Applications for renewable energy conversion and storage," Renewable and Sustainable Energy Reviews, Elsevier, vol. 145(C).
    2. Xu, Bin & Lee, Jinwoo & Kwon, Daeil & Kong, Lingxi & Pecht, Michael, 2021. "Mitigation strategies for Li-ion battery thermal runaway: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 150(C).

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