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Band structure engineered layered metals for low-loss plasmonics

Author

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  • Morten N. Gjerding

    (Center for Atomic-scale Materials Design (CAMD), Technical University of Denmark
    Center for Nanostructured Graphene (CNG), Technical University of Denmark)

  • Mohnish Pandey

    (Center for Atomic-scale Materials Design (CAMD), Technical University of Denmark)

  • Kristian S. Thygesen

    (Center for Atomic-scale Materials Design (CAMD), Technical University of Denmark
    Center for Nanostructured Graphene (CNG), Technical University of Denmark)

Abstract

Plasmonics currently faces the problem of seemingly inevitable optical losses occurring in the metallic components that challenges the implementation of essentially any application. In this work, we show that Ohmic losses are reduced in certain layered metals, such as the transition metal dichalcogenide TaS2, due to an extraordinarily small density of states for scattering in the near-IR originating from their special electronic band structure. On the basis of this observation, we propose a new class of band structure engineered van der Waals layered metals composed of hexagonal transition metal chalcogenide-halide layers with greatly suppressed intrinsic losses. Using first-principles calculations, we show that the suppression of optical losses lead to improved performance for thin-film waveguiding and transformation optics.

Suggested Citation

  • Morten N. Gjerding & Mohnish Pandey & Kristian S. Thygesen, 2017. "Band structure engineered layered metals for low-loss plasmonics," Nature Communications, Nature, vol. 8(1), pages 1-8, April.
  • Handle: RePEc:nat:natcom:v:8:y:2017:i:1:d:10.1038_ncomms15133
    DOI: 10.1038/ncomms15133
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    Cited by:

    1. Shufeng Kong & Francesco Ricci & Dan Guevarra & Jeffrey B. Neaton & Carla P. Gomes & John M. Gregoire, 2022. "Density of states prediction for materials discovery via contrastive learning from probabilistic embeddings," Nature Communications, Nature, vol. 13(1), pages 1-12, December.

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