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Ultrahigh-resolution imaging of water networks by atomic force microscopy

Author

Listed:
  • Akitoshi Shiotari

    (The University of Tokyo)

  • Yoshiaki Sugimoto

    (The University of Tokyo)

Abstract

Local defects in water layers growing on metal surfaces have a key influence on the wetting process at the surfaces; however, such minor structures are undetectable by macroscopic methods. Here, we demonstrate ultrahigh-resolution imaging of single water layers on a copper(110) surface by using non-contact atomic force microscopy (AFM) with molecular functionalized tips at 4.8 K. AFM with a probe tip terminated by carbon monoxide predominantly images oxygen atoms, whereas the contribution of hydrogen atoms is modest. Oxygen skeletons in the AFM images reveal that the water networks containing local defects and edges are composed of pentagonal and hexagonal rings. The results reinforce the applicability of AFM to characterize atomic structures of weakly bonded molecular assemblies.

Suggested Citation

  • Akitoshi Shiotari & Yoshiaki Sugimoto, 2017. "Ultrahigh-resolution imaging of water networks by atomic force microscopy," Nature Communications, Nature, vol. 8(1), pages 1-7, April.
    • Handle: RePEc:nat:natcom:v:8:y:2017:i:1:d:10.1038_ncomms14313
    DOI: 10.1038/ncomms14313
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    Cited by:

    1. Ye Tian & Botao Huang & Yizhi Song & Yirui Zhang & Dong Guan & Jiani Hong & Duanyun Cao & Enge Wang & Limei Xu & Yang Shao-Horn & Ying Jiang, 2024. "Effect of ion-specific water structures at metal surfaces on hydrogen production," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    2. Kuichang Zuo & Xiang Zhang & Xiaochuan Huang & Eliezer F. Oliveira & Hua Guo & Tianshu Zhai & Weipeng Wang & Pedro J. J. Alvarez & Menachem Elimelech & Pulickel M. Ajayan & Jun Lou & Qilin Li, 2022. "Ultrahigh resistance of hexagonal boron nitride to mineral scale formation," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    3. Pengcheng Chen & Qiuhao Xu & Zijing Ding & Qing Chen & Jiyu Xu & Zhihai Cheng & Xiaohui Qiu & Bingkai Yuan & Sheng Meng & Nan Yao, 2023. "Identification of a common ice nucleus on hydrophilic and hydrophobic close-packed metal surfaces," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

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