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Planar-integrated single-crystalline perovskite photodetectors

Author

Listed:
  • Makhsud I. Saidaminov

    (Solar and Photovoltaics Engineering Center, King Abdullah University of Science and Technology (KAUST))

  • Valerio Adinolfi

    (University of Toronto)

  • Riccardo Comin

    (University of Toronto)

  • Ahmed L. Abdelhady

    (Solar and Photovoltaics Engineering Center, King Abdullah University of Science and Technology (KAUST))

  • Wei Peng

    (Solar and Photovoltaics Engineering Center, King Abdullah University of Science and Technology (KAUST))

  • Ibrahim Dursun

    (Solar and Photovoltaics Engineering Center, King Abdullah University of Science and Technology (KAUST))

  • Mingjian Yuan

    (University of Toronto)

  • Sjoerd Hoogland

    (University of Toronto)

  • Edward H. Sargent

    (University of Toronto)

  • Osman M. Bakr

    (Solar and Photovoltaics Engineering Center, King Abdullah University of Science and Technology (KAUST))

Abstract

Hybrid perovskites are promising semiconductors for optoelectronic applications. However, they suffer from morphological disorder that limits their optoelectronic properties and, ultimately, device performance. Recently, perovskite single crystals have been shown to overcome this problem and exhibit impressive improvements: low trap density, low intrinsic carrier concentration, high mobility, and long diffusion length that outperform perovskite-based thin films. These characteristics make the material ideal for realizing photodetection that is simultaneously fast and sensitive; unfortunately, these macroscopic single crystals cannot be grown on a planar substrate, curtailing their potential for optoelectronic integration. Here we produce large-area planar-integrated films made up of large perovskite single crystals. These crystalline films exhibit mobility and diffusion length comparable with those of single crystals. Using this technique, we produced a high-performance light detector showing high gain (above 104 electrons per photon) and high gain-bandwidth product (above 108 Hz) relative to other perovskite-based optical sensors.

Suggested Citation

  • Makhsud I. Saidaminov & Valerio Adinolfi & Riccardo Comin & Ahmed L. Abdelhady & Wei Peng & Ibrahim Dursun & Mingjian Yuan & Sjoerd Hoogland & Edward H. Sargent & Osman M. Bakr, 2015. "Planar-integrated single-crystalline perovskite photodetectors," Nature Communications, Nature, vol. 6(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:6:y:2015:i:1:d:10.1038_ncomms9724
    DOI: 10.1038/ncomms9724
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    Cited by:

    1. Riccardo Ollearo & Junke Wang & Matthew J. Dyson & Christ H. L. Weijtens & Marco Fattori & Bas T. Gorkom & Albert J. J. M. Breemen & Stefan C. J. Meskers & René A. J. Janssen & Gerwin H. Gelinck, 2021. "Ultralow dark current in near-infrared perovskite photodiodes by reducing charge injection and interfacial charge generation," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    2. Rohit Abraham John & Yiğit Demirağ & Yevhen Shynkarenko & Yuliia Berezovska & Natacha Ohannessian & Melika Payvand & Peng Zeng & Maryna I. Bodnarchuk & Frank Krumeich & Gökhan Kara & Ivan Shorubalko &, 2022. "Reconfigurable halide perovskite nanocrystal memristors for neuromorphic computing," Nature Communications, Nature, vol. 13(1), pages 1-10, December.

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