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Elastic, strong and tough ionically conductive elastomers

Author

Listed:
  • Burebi Yiming

    (PSL University
    Zhejiang University)

  • Simon Hubert

    (PSL University)

  • Alex Cartier

    (PSL University)

  • Bruno Bresson

    (PSL University)

  • Gabriel Mello

    (PSL University)

  • Armelle Ringuede

    (PSL University)

  • Costantino Creton

    (PSL University)

Abstract

Stretchable elastic materials with high strength, toughness, and good ionic conductivity are highly desirable for wearable devices and stretchable batteries. Unfortunately, limited success has been reported to attain all of these properties simultaneously. Here, we report a family of ionically conductive elastomers (ICEs) without compromise between mechanical properties (high stiffness, reversible elasticity, fracture resistance) and ionic conductivity, by introducing a multiple network elastomer (MNE) architecture into a low $${T}_{g}$$ T g polymer. The ICEs with the MNE architecture exhibit a room temperature ionic conductivity of the order of $${10}^{-6}\,{{{\rm{S}}}.{{\rm{cm}}}}^{-1}$$ 10 − 6 S . cm − 1 and stress at break of ~8 MPa, whereas the simple networks without an MNE architecture show two orders magnitude lower ionic conductivity ( $${10}^{-8}\,{{{\rm{S}}}.{{\rm{cm}}}}^{-1}$$ 10 − 8 S . cm − 1 ) and comparably low strength (

Suggested Citation

  • Burebi Yiming & Simon Hubert & Alex Cartier & Bruno Bresson & Gabriel Mello & Armelle Ringuede & Costantino Creton, 2025. "Elastic, strong and tough ionically conductive elastomers," Nature Communications, Nature, vol. 16(1), pages 1-11, December.
  • Handle: RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-024-55472-8
    DOI: 10.1038/s41467-024-55472-8
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    References listed on IDEAS

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    1. Lei Shi & Tianxiang Zhu & Guoxin Gao & Xinyu Zhang & Wei Wei & Wenfeng Liu & Shujiang Ding, 2018. "Highly stretchable and transparent ionic conducting elastomers," Nature Communications, Nature, vol. 9(1), pages 1-7, December.
    2. Zhouyue Lei & Peiyi Wu, 2019. "A highly transparent and ultra-stretchable conductor with stable conductivity during large deformation," Nature Communications, Nature, vol. 10(1), pages 1-9, December.
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