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Long-term reliable wireless H2 gas sensor via repeatable thermal refreshing of palladium nanowire

Author

Listed:
  • Ki-Hoon Kim

    (Pusan National University)

  • Min-Seung Jo

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Sung-Ho Kim

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Bokyeong Kim

    (Pusan National University)

  • Joonhee Kang

    (Pusan National University)

  • Jun-Bo Yoon

    (Korea Advanced Institute of Science and Technology (KAIST))

  • Min-Ho Seo

    (Pusan National University
    Pusan National University)

Abstract

The increasing significance of hydrogen (H2) gas as a clean energy source has prompted the development of high-performance H2 gas sensors. Palladium (Pd)-based sensors, with their advantages of selectivity, scalability, and cost-effectiveness, have shown promise in this regard. However, the long-term stability and reliability of Pd-based sensors remain a challenge. This study not only identifies the exact cause for performance degradation in palladium (Pd) nanowire H2 sensors, but also implements and optimizes a cost-effective recovery method. The results from density functional theory (DFT) calculations and material analysis confirm the presence of C = O bonds, indicating performance degradation due to carbon dioxide (CO2) accumulation on the Pd surface. Based on the molecular behavior calculation in high temperatures, we optimized the thermal treatment method of 200 °C for 10 minutes to remove the C = O contaminants, resulting in nearly 100% recovery of the sensor’s initial performance even after 2 months of contamination.

Suggested Citation

  • Ki-Hoon Kim & Min-Seung Jo & Sung-Ho Kim & Bokyeong Kim & Joonhee Kang & Jun-Bo Yoon & Min-Ho Seo, 2024. "Long-term reliable wireless H2 gas sensor via repeatable thermal refreshing of palladium nanowire," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-53080-0
    DOI: 10.1038/s41467-024-53080-0
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    1. Baroutaji, Ahmad & Wilberforce, Tabbi & Ramadan, Mohamad & Olabi, Abdul Ghani, 2019. "Comprehensive investigation on hydrogen and fuel cell technology in the aviation and aerospace sectors," Renewable and Sustainable Energy Reviews, Elsevier, vol. 106(C), pages 31-40.
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