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Multipole engineering by displacement resonance: a new degree of freedom of Mie resonance

Author

Listed:
  • Yu-Lung Tang

    (National Taiwan University)

  • Te-Hsin Yen

    (National Taiwan University)

  • Kentaro Nishida

    (National Taiwan University)

  • Chien-Hsuan Li

    (National Taiwan University)

  • Yu-Chieh Chen

    (National Taiwan University)

  • Tianyue Zhang

    (Jinan University)

  • Chi-Kang Pai

    (National Taiwan University)

  • Kuo-Ping Chen

    (National Yang Ming Chiao Tung University
    National Tsing Hua University)

  • Xiangping Li

    (Jinan University)

  • Junichi Takahara

    (Osaka University
    Osaka University)

  • Shi-Wei Chu

    (National Taiwan University
    National Taiwan University
    National Tsing Hua University)

Abstract

The canonical studies on Mie scattering unravel strong electric/magnetic optical responses in nanostructures, laying foundation for emerging meta-photonic applications. Conventionally, the morphology-sensitive resonances hinge on the normalized frequency, i.e. particle size over wavelength, but non-paraxial incidence symmetry is overlooked. Here, through confocal reflection microscopy with a tight focus scanning over silicon nanostructures, the scattering point spread functions unveil distinctive spatial patterns featuring that linear scattering efficiency is maximal when the focus is misaligned. The underlying physical mechanism is the excitation of higher-order multipolar modes, not accessible by plane wave irradiation, via displacement resonance, which showcases a significant reduction of nonlinear response threshold, sign flip in all-optical switching, and spatial resolution enhancement. Our result fundamentally extends the century-old light scattering theory, and suggests new dimensions to tailor Mie resonances.

Suggested Citation

  • Yu-Lung Tang & Te-Hsin Yen & Kentaro Nishida & Chien-Hsuan Li & Yu-Chieh Chen & Tianyue Zhang & Chi-Kang Pai & Kuo-Ping Chen & Xiangping Li & Junichi Takahara & Shi-Wei Chu, 2023. "Multipole engineering by displacement resonance: a new degree of freedom of Mie resonance," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-43063-y
    DOI: 10.1038/s41467-023-43063-y
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    References listed on IDEAS

    as
    1. Yi-Shiou Duh & Yusuke Nagasaki & Yu-Lung Tang & Pang-Han Wu & Hao-Yu Cheng & Te-Hsin Yen & Hou-Xian Ding & Kentaro Nishida & Ikuto Hotta & Jhen-Hong Yang & Yu-Ping Lo & Kuo-Ping Chen & Katsumasa Fujit, 2020. "Giant photothermal nonlinearity in a single silicon nanostructure," Nature Communications, Nature, vol. 11(1), pages 1-9, December.
    2. Yi-Shiou Duh & Yusuke Nagasaki & Yu-Lung Tang & Pang-Han Wu & Hao-Yu Cheng & Te-Hsin Yen & Hou-Xian Ding & Kentaro Nishida & Ikuto Hotta & Jhen-Hong Yang & Yu-Ping Lo & Kuo-Ping Chen & Katsumasa Fujit, 2020. "Publisher Correction: Giant photothermal nonlinearity in a single silicon nanostructure," Nature Communications, Nature, vol. 11(1), pages 1-1, December.
    3. B. le Feber & N. Rotenberg & L. Kuipers, 2015. "Nanophotonic control of circular dipole emission," Nature Communications, Nature, vol. 6(1), pages 1-6, November.
    4. Martin Neugebauer & Paweł Woźniak & Ankan Bag & Gerd Leuchs & Peter Banzer, 2016. "Polarization-controlled directional scattering for nanoscopic position sensing," Nature Communications, Nature, vol. 7(1), pages 1-6, September.
    5. Tianyue Zhang & Ying Che & Kai Chen & Jian Xu & Yi Xu & Te Wen & Guowei Lu & Xiaowei Liu & Bin Wang & Xiaoxuan Xu & Yi-Shiou Duh & Yu-Lung Tang & Jing Han & Yaoyu Cao & Bai-Ou Guan & Shi-Wei Chu & Xia, 2020. "Anapole mediated giant photothermal nonlinearity in nanostructured silicon," Nature Communications, Nature, vol. 11(1), pages 1-9, December.
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