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Unveiling the double-peak structure of quantum oscillations in the specific heat

Author

Listed:
  • Zhuo Yang

    (The University of Tokyo)

  • Benoît Fauqué

    (PSL Research University)

  • Toshihiro Nomura

    (The University of Tokyo)

  • Takashi Shitaokoshi

    (The University of Tokyo)

  • Sunghoon Kim

    (Cornell University)

  • Debanjan Chowdhury

    (Cornell University)

  • Zuzana Pribulová

    (Slovak Academy of Sciences)

  • Jozef Kačmarčík

    (Slovak Academy of Sciences)

  • Alexandre Pourret

    (Univ. Grenoble Alpes, CEA, Grenoble INP, IRIG, PHELIQS)

  • Georg Knebel

    (Univ. Grenoble Alpes, CEA, Grenoble INP, IRIG, PHELIQS)

  • Dai Aoki

    (Tohoku University, Oarai)

  • Thierry Klein

    (Univ. Grenoble Alpes, CNRS, Institut Néel)

  • Duncan K. Maude

    (Laboratoire National des Champs Magnétiques Intenses, CNRS-UGA-UPS-INSA)

  • Christophe Marcenat

    (Univ. Grenoble Alpes, CEA, Grenoble INP, IRIG, PHELIQS)

  • Yoshimitsu Kohama

    (The University of Tokyo)

Abstract

Quantum oscillation phenomenon is an essential tool to understand the electronic structure of quantum matter. Here we report a systematic study of quantum oscillations in the electronic specific heat Cel in natural graphite. We show that the crossing of a single spin Landau level and the Fermi energy give rise to a double-peak structure, in striking contrast to the single peak expected from Lifshitz-Kosevich theory. Intriguingly, the double-peak structure is predicted by the kernel term for Cel/T in the free electron theory. The Cel/T represents a spectroscopic tuning fork of width 4.8kBT which can be tuned at will to resonance. Using a coincidence method, the double-peak structure can be used to accurately determine the Landé g-factors of quantum materials. More generally, the tuning fork can be used to reveal any peak in fermionic density of states tuned by magnetic field, such as Lifshitz transition in heavy-fermion compounds.

Suggested Citation

  • Zhuo Yang & Benoît Fauqué & Toshihiro Nomura & Takashi Shitaokoshi & Sunghoon Kim & Debanjan Chowdhury & Zuzana Pribulová & Jozef Kačmarčík & Alexandre Pourret & Georg Knebel & Dai Aoki & Thierry Klei, 2023. "Unveiling the double-peak structure of quantum oscillations in the specific heat," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-42730-4
    DOI: 10.1038/s41467-023-42730-4
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    References listed on IDEAS

    as
    1. B. Michon & C. Girod & S. Badoux & J. Kačmarčík & Q. Ma & M. Dragomir & H. A. Dabkowska & B. D. Gaulin & J.-S. Zhou & S. Pyon & T. Takayama & H. Takagi & S. Verret & N. Doiron-Leyraud & C. Marcenat & , 2019. "Thermodynamic signatures of quantum criticality in cuprate superconductors," Nature, Nature, vol. 567(7747), pages 218-222, March.
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