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Complex-tensor theory of simple smectics

Author

Listed:
  • Jack Paget

    (Loughborough University)

  • Marco G. Mazza

    (Loughborough University
    Max Planck Institute for Dynamics and Self-Organization (MPIDS))

  • Andrew J. Archer

    (Loughborough University)

  • Tyler N. Shendruk

    (The University of Edinburgh)

Abstract

Matter self-assembling into layers generates unique properties, including structures of stacked surfaces, directed transport, and compact area maximization that can be highly functionalized in biology and technology. Smectics represent the paradigm of such lamellar materials — they are a state between fluids and solids, characterized by both orientational and partial positional ordering in one layering direction, making them notoriously difficult to model, particularly in confining geometries. We propose a complex tensor order parameter to describe the local degree of lamellar ordering, layer displacement and orientation of the layers for simple, lamellar smectics. The theory accounts for both dislocations and disclinations, by regularizing singularities within defect cores and so remaining continuous everywhere. The ability to describe disclinations and dislocation allows this theory to simulate arrested configurations and inclusion-induced local ordering. This tensorial theory for simple smectics considerably simplifies numerics, facilitating studies on the mesoscopic structure of topologically complex systems.

Suggested Citation

  • Jack Paget & Marco G. Mazza & Andrew J. Archer & Tyler N. Shendruk, 2023. "Complex-tensor theory of simple smectics," Nature Communications, Nature, vol. 14(1), pages 1-13, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-36506-z
    DOI: 10.1038/s41467-023-36506-z
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    References listed on IDEAS

    as
    1. P. Guillamat & J. Ignés-Mullol & F. Sagués, 2017. "Taming active turbulence with patterned soft interfaces," Nature Communications, Nature, vol. 8(1), pages 1-8, December.
    2. René Wittmann & Louis B. G. Cortes & Hartmut Löwen & Dirk G. A. L. Aarts, 2021. "Particle-resolved topological defects of smectic colloidal liquid crystals in extreme confinement," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
    3. Xu, Aiguo & Gonnella, G. & Lamura, A., 2004. "Numerical study of the ordering properties of lamellar phase," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 344(3), pages 750-756.
    4. S. M. Hashemi & U. Jagodič & M. R. Mozaffari & M. R. Ejtehadi & I. Muševič & M. Ravnik, 2017. "Fractal nematic colloids," Nature Communications, Nature, vol. 8(1), pages 1-9, April.
    5. Min-Jun Gim & Daniel A. Beller & Dong Ki Yoon, 2017. "Morphogenesis of liquid crystal topological defects during the nematic-smectic A phase transition," Nature Communications, Nature, vol. 8(1), pages 1-9, August.
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